2025

Analysis of the Electrochemical Stability of Sulfide Solid Electrolyte Dry Films for Improved Dry‐Processed Solid‐State Batteries

M. Rosner, Ş. Cangaz, F. Hippauf, S. Dörfler, B. Aktekin, T. Meyer, A. Henß, T. Abendroth, H. Althues, J. Janek, S. Kaskel

Advanced Functional Materials, 2025, 36 17, DOI: 10.1002/adfm.202518517

Assessing the Impact of Li+ Concentration and Stacking Faults in the Aliovalent-Substituted Ionic Conductor Li3ScCl6

C. Rosenbach, B. Helm, E. Suard, B. V. Lotsch, S. Bette, W. G. Zeier

Inorganic Chemistry, 2025, 64 25, 12698-12707 DOI: 10.1021/acs.inorgchem.5c01371

Attaining a fast-conducting, hybrid solid state separator for all solid-state batteries through a facile wet infiltration method

P. Heuer, L. Ketter, M. Rana, F. Scharf, G. Brunklaus, W. G. Zeier

Energy Advances, 2025, 4 11, 1356-1362 DOI: 10.1039/d5ya00141b

Blend Electrodes in Lithium‐Ion Batteries: Investigation of Inhomogeneities Using a Spatially Resolved Transmission Line Model

M. Schamel, J. Knorr, A. Kinberger, M. A. Danzer

Batteries & Supercaps, 2025, 8 11, DOI: 10.1002/batt.202500147

Ceramic-Rich Composite Separators for High-Voltage Solid-State Batteries

K. Vattappara, M. Finsterbusch, D. Fattakhova‐Rohlfing, I. Urdampilleta, A. Kvasha

Batteries, 2025, 11 2, 42 DOI: 10.3390/batteries11020042

Chemical and Structural Degradation of Single Crystalline High‐Nickel Cathode Materials During High‐Voltage Holds

K. Vettori, S. Schröder, L. Ahrens, R. Wilhelm, S. Kremer, J. K. Eckhardt, T. Brezesinski, A. Kondrakov, J. Mayer, A. Henß, J. Janek

Advanced Energy Materials, 2025, 15 33, DOI: 10.1002/aenm.202502148

Chemo-thermal stress in all-solid-state batteries: Impact of cathode active materials and microstructure

F. Al‐Jaljouli, R. Mücke, C. Roitzheim, Y. J. Sohn, N. Yaqoob, M. Finsterbusch, P. Kaghazchi, O. Guillon

Journal of Power Sources, 2025, 644 , 237136 DOI: 10.1016/j.jpowsour.2025.237136

Correction to “Correlation between the Coherence Length and Ionic Conductivity in LiNbOCl 4 via the Anion Stoichiometry”

J. A. Newnham, J. Kondek, J. Härtel, C. Rosenbach, C. Li, V. Faka, L. M. Gronych, D. Glikman, F. Schreiner, D. D. Wind, B. Braunschweig, M. R. Hansen, W. G. Zeier

Chemistry of Materials, 2025, 37 20, 8472 DOI: 10.1021/acs.chemmater.5c02304

Correlation between the Coherence Length and Ionic Conductivity in LiNbOCl4 via the Anion Stoichiometry

J. A. Newnham, J. Kondek, J. Härtel, C. Rosenbach, C. Li, V. Faka, L. M. Gronych, D. Glikman, F. Schreiner, D. D. Wind, B. Braunschweig, M. R. Hansen, W. G. Zeier

Chemistry of Materials, 2025, 37 11, 4130-4144 DOI: 10.1021/acs.chemmater.5c00627

Crosslinked ionogels containing a Li-conducting inorganic phase as electrolyte for lithium-metal batteries

M. Gandolfo, M. Longo, T. Diemant, S. Bodoardo, D. Bresser, J. Amici

Journal of Energy Chemistry, 2025, 107 , 221-232 DOI: 10.1016/j.jechem.2025.03.056

Dry Battery Electrode Technology: From Early Concepts to Industrial Applications

B. Schumm, A. Dupuy, M. Lux, C. Girsule, S. Dörfler, F. Schmidt, M. Fiedler, M. Rosner, F. Hippauf, S. Kaskel

Advanced Energy Materials, 2025, 15 24, DOI: 10.1002/aenm.202406011

Effect of Stack Pressure on the Microstructure and Ionic Conductivity of the Slurry‐Processed Solid Electrolyte Li 7 SiPS 8

D. H. Nguyen, M. Osenberg, C. Schneider, J. Moosmann, F. Beckmann, I. Manke, B. V. Lotsch

Advanced Materials Interfaces, 2025, 12 24, DOI: 10.1002/admi.202500845

Effect of a Two-Step Temperature-Swing Synthesis on Coarse-Grained LiNiO2 Secondary Particles Characterized by Scanning Transmission Electron Microscopy

T. Demuth, P. Kurzhals, S. Ahmed, F. Riewald, M. Malaki, J. Haust, A. Beyer, J. Janek, K. Volz

Chemistry of Materials, 2025, 37 11, 3993-4004 DOI: 10.1021/acs.chemmater.5c00108

Effect of particle size on the slurry-based processability and conductivity of t -Li 7 SiPS 8

D. H. Nguyen, L. Grunenberg, I. Moudrakovski, K. Küster, B. V. Lotsch

EES batteries., 2025, 1 4, 824-832 DOI: 10.1039/d5eb00005j

Elemental Segregation at LLZO Grain Boundaries: Eliminating Its Detrimental Role in Conductivity and Lithium Nucleation

D. Fattakhova‐Rohlfing, K. Yao, K. Kim, D. Jennings, J. Dippell, M. Ma, X. Liu, Q. Ma, W. S. Scheld, C. Roitzheim, Y. Zeng, T. Danner, O. Guillon, M. Huijben, J. E. ten Elshof, L. F. Wan, A. Latz, B. C. Wood, M. Finsterbusch

Research Square, 2025,  , DOI: 10.21203/rs.3.rs-7887285/v1

Enabling high mass loadings for polymer based all solid-state batteries with temperature assisted solvent-free vacuum melt infiltration

A. Buchheit, F. Scharf, S. Krämer, M. Grünebaum, M. Winter, G. Brunklaus

Energy storage materials, 2025, 83 , 104670 DOI: 10.1016/j.ensm.2025.104670

Enhancing Transparency: Reporting data reliability in prospective assessments of emerging battery technologies

S. Weber-Harmann, K. Fischer, N. Kononova, N. Dilger, J. Baars, S. Zellmer, C. S. Herrmann

Procedia CIRP, 2025, 135 , 1271-1276 DOI: 10.1016/j.procir.2025.03.005

Equilibration of ion distribution at polymer/ceramic interfaces

M. Kozdra, L. Hoelzer, D. Brandell, A. Heuer

Physical Chemistry Chemical Physics, 2025, 27 46, 24918-24931 DOI: 10.1039/d5cp01988e

Evolution, Collapse, and Recovery of Electronically Conductive Networks in Sulfide‐Based All‐Solid‐State Batteries Using Passivation‐Coated NMC and C65

N. Papadopoulos, E. Reisacher, T. Schubert, S. Hein, T. Danner, A. Latz, P. Kaya, V. Knoblauch

Batteries & Supercaps, 2025, 8 12, DOI: 10.1002/batt.202500321

Fast‐Charging of Solid‐State Batteries Enabled by Functional Additives Infused into High‐Mass‐Loading Nickel Manganese Cobalt Cathodes

P. Glomb, M. M. Mitchell, L. Wichmann, N. Tänzer, M. Winter, G. Brunklaus

Batteries & Supercaps, 2025, 9 3, DOI: 10.1002/batt.202500679

Fluorine-free polysiloxane-based single-ion-conducting polymer electrolyte for lithium–metal batteries

L. Gräber, V. Marangon, M. Kumar, M. Weil, D. Bresser

Green Chemistry, 2025, 27 27, 8226-8236 DOI: 10.1039/d5gc00252d

Formation, Growth, and Shrinkage of Voids in Lithium Metal in Contact With an LLZO Electrolyte

S. Lang, L. Hennerici, D. Kramer, D. Avadanii, S. Mück, M. Linz, J. Kita, R. Moos, R. Mönig

ACS Applied Materials & Interfaces, 2025, 17 41, 56980-56990 DOI: 10.1021/acsami.5c09594

Graded Cathode Design for Enhanced Performance of Sulfide-Based Solid-State Batteries

E. Schlautmann, J. Drews, L. Ketter, M. Lange, T. Danner, A. Latz, W. G. Zeier

ACS Energy Letters, 2025, 10 4, 1664-1670 DOI: 10.1021/acsenergylett.4c03243

High-rate performance solid-state lithium batteries achieved by infiltrating a single-layer LLZO scaffold

M. Zubair, R. Ye, X. Liu, K. Touidjine, P. V. Soundaraj, M. Finsterbusch, F. Tietz, D. Fattakhova-Rohlfing, O. Guillon

Journal of Power Sources, 2025, 666 , 239065 DOI: 10.1016/j.jpowsour.2025.239065

In Situ 4D STEM of LiNiO 2 Particles Heated in an Oxygen Atmosphere: Toward Investigation of Solid‐State Batteries Under Realistic Processing Conditions

T. Demuth, S. Ahmed, P. Kurzhals, J. Haust, J. Belz, A. Beyer, J. Janek, K. Volz

Small Methods, 2025, 10 2, e2500357 DOI: 10.1002/smtd.202500357

Increasing the cycling stability of LLZO-based solid-state batteries with Li3BO3 as catholyte

W. S. Scheld, Y. Collette, K. Touidjine, C. Roitzheim, Y. J. Sohn, D. Fattakhova‐Rohlfing

Journal of Power Sources, 2025, 652 , 237322 DOI: 10.1016/j.jpowsour.2025.237322

LISA: A Lithium-Ion Solid-State Assistant using large language models for knowledge defragmentation in battery science and beyond

Y. Zhao, A. Hansen, A. Dahlhaus, N. Brandt, M. Selzer, A. Koeppe, B. Nestler, M. Knapp, H. Ehrenberg

Materials Today Communications, 2025, 45 , 112380 DOI: 10.1016/j.mtcomm.2025.112380

LiI-Modified Glass-Ceramic Lithium Thioborate: From Fundamentals to Applications in Solid-State Batteries

S. E. Holmes, J. Kondek, P. Zhang, V. Faka, J. A. Newnham, L. M. Gronych, M. R. Hansen, W. G. Zeier, Y. Cui

Chemistry of Materials, 2025, 37 7, 2642-2649 DOI: 10.1021/acs.chemmater.5c00224

LiNbO 3 Coatings on NCM622: Structure and Performance Insights

J. Haust, Y. Guo, J. Belz, S. Ahmed, N. Adeli, F. Hüppe, L. C. Erhard, V. Mereacre, J. Rohrer, A. Hansen, H. Ehrenberg, K. Albe, J. R. Binder, K. Volz

Advanced Materials Interfaces, 2025, 12 17, DOI: 10.1002/admi.202500590

Material-Adapted Gripping and Handling of PEO-Based Cell Components for All-Solid-State Battery Cell Stacking

D. M. Nguyen, T. Scharmann, K. Dröder

N/A, 2025,  , 111-122 DOI: 10.1007/978-3-031-74010-7_10

Microstructure of Silicon Anodes in Solid‐State Batteries ‐ From Crystalline to Amorphous

S. Ahmed, F. Rossi, H. Huo, J. Haust, F. Hüppe, J. Belz, A. Beyer, J. Janek, K. Volz

Advanced Energy Materials, 2025, 16 2, DOI: 10.1002/aenm.202504418

Modeling chemo-thermal mechanical stresses in all-solid-state lithium Batteries: Influence of grain morphology and alignment

F. Al‐Jaljouli, R. Mücke, M. Finsterbusch, P. Kaghazchi, O. Guillon

Journal of Power Sources, 2025, 653 , 237539 DOI: 10.1016/j.jpowsour.2025.237539

Progress and Challenges in Li M OCl 4 and Na M OCl 4 ( M = Nb, Ta) Oxyhalide Solid Electrolytes for Solid‐State Batteries

J. A. Newnham, A. G. Squires, M. A. Kraft, D. O. Scanlon, W. G. Zeier

Advanced Energy Materials, 2025, 15 43, DOI: 10.1002/aenm.202504067

Purity of lithium metal electrode and its impact on lithium stripping in solid-state batteries

J. Becker, T. Weintraut, S. L. Benz, T. Fuchs, C. Lerch, P. Becker, J. K. Eckhardt, A. Henß, F. H. Richter, J. Janek

Nature Communications, 2025, 16 1, 5395 DOI: 10.1038/s41467-025-61006-7

Quantifying the Impact of Cathode Composite Mixing Quality on Active Mass Utilization and Reproducibility of Solid‐State Battery Cells

M. Kissel, M. Schosland, J. Töws, D. Kalita, Y. Schneider, J. Kessler‐Kühn, S. Schröder, J. Schubert, F. Frankenberg, A. Kwade, A. Bielefeld, F. H. Richter, J. Janek

Advanced Energy Materials, 2025, 15 27, DOI: 10.1002/aenm.202405405

Revisiting polymer coatings on nanoparticles: correlation between molecular weight and coating thickness in chain transfer polymerizations

D. Döpping, A. Stihl, D. Voll, F. H. Schacher, P. Théato

Polymer Chemistry, 2025, 16 18, 2075-2082 DOI: 10.1039/d5py00081e

Rotational Stacking Faults in the Ionic Conductor Li 3 ScCl 6

B. A. Goldmann, C. Rosenbach, H. A. Evans, B. Helm, B. Wankmiller, O. Maus, E. Suard, L. F. Nazar, M. R. Hansen, B. J. Morgan, M. S. Islam, W. G. Zeier

Chemistry of Materials, 2025, 37 24, 9858-9868 DOI: 10.1021/acs.chemmater.5c02303

Scalable cathode electrode and sulfidic separator manufacturing by DRYtraec® process for solid-state batteries

A. Dupuy, Ş. Cangaz, M. Rosner, F. Hippauf, T. Abendbroth, H. Althues, S. Kaskel, B. Schumm

Journal of Energy Storage, 2025, 134 , 118172 DOI: 10.1016/j.est.2025.118172

Structural Analysis of Tin-Substituted High-Entropy Li-Garnet Electrolytes for Solid-State Batteries

B. Zimmermann, T. Fuchs, J. A. Westphal, J. Janek, M. Lepple

ACS Organic & Inorganic Au, 2025, 5 3, 211-220 DOI: 10.1021/acsorginorgau.5c00021

Structure and Transport Properties in the Pseudobinary Phase System Li4SiS4–Li4SnS4

L. G. Balzat, Y. Li, S. Dums, I. Moudrakovski, K. Gjorgjevikj, A. Schulz, Y. Li, S. Krause, P. Canepa, B. V. Lotsch

Chemistry of Materials, 2025, 37 16, 6127-6139 DOI: 10.1021/acs.chemmater.5c00358

Structure and transport properties in the pseudo-binary phase system Li4SiS4 – Li4SnS4

L. G. Balzat, Y. Li, S. Dums, I. Moudrakovski, K. Gjorgjevikj, A. Schulz, Y. Li, S. Krause, P. Canepa, B. V. Lotsch

ChemRxiv, 2025,  , DOI: 10.26434/chemrxiv-2025-bssbr

Temperature and concentration dependence of the ionic charge transfer between solid and liquid Li+ electrolytes – the systems LLZO:Ta/LiPF6–EC–DMC, LATP/LiPF6–EC–DMC and LLZO:Ta/LiBOB–DME–THF

T. Wekking, M. Finsterbusch, C. Korte

Physical Chemistry Chemical Physics, 2025, 27 11, 5543-5554 DOI: 10.1039/d4cp04738a

Toward Higher Energy Density All‐Solid‐State Batteries by Production of Freestanding Thin Solid Sulfidic Electrolyte Membranes in a Roll‐to‐Roll Process

M. Rosner, Ş. Cangaz, A. Dupuy, F. Hippauf, S. Dörfler, T. Abendroth, B. Schumm, H. Althues, S. Kaskel

Advanced Energy Materials, 2025, 15 19, DOI: 10.1002/aenm.202404790

Uni‐Axial Densification of Slurry‐Casted Li₆PS₅Cl Tapes: The Role of Particle Size Distribution and Densification Pressure

Q. A. Tran, M. Agrawal, M. Häusler, J. Hormann, M. Moqadam, G. J. Redhammer, I. S. Ellingsen, M. M. U. Din, P. E. Vullum, R. Zettl, T. Danner, A. Latz, V. Hennige, R. Brunner, D. Rettenwander

Advanced Materials, 2025, 37 30, e2501592 DOI: 10.1002/adma.202501592

Unveiling SEI Formation Dynamics of PEO: LiTFSI with Lithium Metal: An In Situ Approach Combining SIMS, XPS, and CTTA

T. Weintraut, A. Weiß, S. L. Benz, B. Aktekin, J. Sann, A. Henß

Advanced Materials Interfaces, 2025, 12 23, DOI: 10.1002/admi.202500392

Using resistor network models to predict the transport properties of solid-state battery composites

L. Ketter, N. Greb, T. Bernges, W. G. Zeier

Nature Communications, 2025, 16 1, 1411 DOI: 10.1038/s41467-025-56514-5

Versatile Solvent‐Free Synthesis of Composite Polymer Electrolytes for Thin High‐Performance Solid‐State Lithium Metal Batteries

D. Döpping, A. Buchheit, X. Liu, A. Goecke, A. P. Grimm, D. Voll, M. Wilhelm, M. Finsterbusch, M. Winter, G. Brunklaus, P. Théato

Small, 2025, 21 37, e04166 DOI: 10.1002/smll.202504166

2024

A Simple Method for the Study of Heteroionic Interface Impedances in Solid Electrolyte Multilayer Cells Containing LLZO

S. Kremer, R. Rekers, U. Sigar, J. Becker, J. Schubert, J. K. Eckhardt, A. Bielefeld, F. H. Richter, J. Janek

ACS Applied Materials & Interfaces, 2024, 16 33, 44236-44248 DOI: 10.1021/acsami.4c07845

A Super‐Ionic Solid‐State Block Copolymer Electrolyte

D. T. Krause, B. Förster, M. Dulle, S. Krämer, S. Böckmann, C. Mönich, M. R. Hansen, M. Schönhoff, V. Siozios, M. Grünebaum, M. Winter, S. Förster, H. Wiemhöfer

Small, 2024, 20 49, e2404297 DOI: 10.1002/smll.202404297

A U-Net-based self-stitching method for generating periodic grain structures

Y. Ji, A. Koeppe, P. Altschuh, L. Griem, D. Rajagopal, B. Nestler

Physica Scripta, 2024, 99 7, 076010 DOI: 10.1088/1402-4896/ad52cf

A conservative and efficient model for grain boundaries of solid electrolytes in a continuum model for solid-state batteries

S. Sinzig, C. P. Schmidt, W. A. Wall

arXiv (Cornell University), 2024,  , DOI: 10.48550/arxiv.2401.06454

A metallic lithium anode for solid-state batteries with low volume change by utilizing a modified porous carbon host

S. Poetke, T. Boenke, K. Henze, K. Schutjajew, J. Kunigkeit, S. L. Benz, Ş. Cangaz, J. Sann, F. Hippauf, S. Dörfler, T. Abendroth, H. Althues, M. Oschatz, E. Brunner, J. Janek, S. Kaskel

Carbon, 2024, 232 , 119821 DOI: 10.1016/j.carbon.2024.119821

Advanced Single-Ion Conducting Block Copolymer Electrolyte for Safer and Less Costly Lithium–Metal Batteries

D. Xu, A. Mayer, Z. Chen, S. Passerini, D. Bresser

ACS Energy Letters, 2024, 9 11, 5279-5287 DOI: 10.1021/acsenergylett.4c02081

An Electro-Chemo-Mechanic Model Resolving Delamination between Components in Complex Microstructures of Solid-State Batteries

C. P. Schmidt, S. Sinzig, W. A. Wall

Journal of The Electrochemical Society, 2024, 171 10, 100502 DOI: 10.1149/1945-7111/ad76dc

Anaysis of the validity of P2D models for solid-state batteries in a large parameter range

S. Sinzig, C. P. Schmidt, W. A. Wall

arXiv (Cornell University), 2024,  , DOI: 10.48550/arxiv.2408.05771

Benchmarking of Coatings for Cathode Active Materials in Solid-State Batteries Using Surface Analysis and Reference Electrodes

J. Hertle, F. Walther, T. Lombardo, C. Kern, B. Pavlovic, B. Mogwitz, X. Wu, H. Schneider, M. Rohnke, J. Janek

ACS Applied Materials & Interfaces, 2024, 16 7, 9400-9413 DOI: 10.1021/acsami.3c15723

Benchmarking the reproducibility of all-solid-state battery cell performance

S. Puls, E. Nazmutdinova, F. Kalyk, H. M. Woolley, J. F. Thomsen, C. Zhu, A. Fauchier‐Magnan, A. Gautam, M. Gockeln, S. Ham, M. T. Hasan, M. Jeong, D. Hiraoka, J. S. Kim, T. Kutsch, B. Lelotte, P. Minnmann, V. Miß, K. Motohashi, D. L. Nelson, F. Ooms, F. Del Piccolo, C. Plank, M. Rosner, S. E. Sandoval, E. Schlautmann, R. Schuster, D. S. Jolly, Y. Sun, B. S. Vishnugopi, R. Zhang, H. Zheng, P. Adelhelm, T. Brezesinski, P. G. Bruce, M. A. Danzer, M. El Kazzi, H. A. Gasteiger, K. B. Hatzell, A. Hayashi, F. Hippauf, J. Janek, Y. S. Jung, M. T. McDowell, Y. S. Meng, P. P. Mukherjee, S. Ohno, B. Roling, A. Sakuda, J. Schwenzel, X. Sun, C. Villevieille, M. Wagemaker, W. G. Zeier, N. M. Vargas‐Barbosa

Nature Energy, 2024, 9 10, 1310-1320 DOI: 10.1038/s41560-024-01634-3

Comprehension-driven design of advanced multi-block single-ion conducting polymer electrolytes for high-performance lithium-metal batteries

X. Dong, D. Bresser

Journal of Energy Chemistry, 2024, 94 , 357-359 DOI: 10.1016/j.jechem.2024.02.018

Current understanding of electrochemical strain microscopy to visualize ion behavior on the nanoscale

F. Hausen, N. Balke

Current Opinion in Electrochemistry, 2024, 47 , 101562 DOI: 10.1016/j.coelec.2024.101562

Decoupling the Effects of Interface Chemical Degradation and Mechanical Cracking in Solid‐State Batteries with Silicon Electrode

H. Huo, Y. Bai, S. L. Benz, T. Weintraut, S. Wang, A. Henß, D. Raabe, J. Janek

Advanced Materials, 2024, 37 7, e2415006 DOI: 10.1002/adma.202415006

Degradation of Styrene-Poly(ethylene oxide)-Based Block Copolymer Electrolytes at the Na and K Negative Electrode Studied by Microcalorimetry and Impedance Spectroscopy

S. Xing, A. D. Khudyshkina, U. Rauska, A. J. Butzelaar, D. Voll, P. Théato, J. Tübke, F. Jeschull

Journal of The Electrochemical Society, 2024, 171 4, 040516 DOI: 10.1149/1945-7111/ad3b72

Direct Precursor Route for the Fabrication of LLZO Composite Cathodes for Solid‐State Batteries

V. Kiyek, C. Schwab, W. S. Scheld, C. Roitzheim, A. Lindner, W. Menesklou, M. Finsterbusch, D. Fattakhova‐Rohlfing, O. Guillon

Advanced Science, 2024, 11 42, e2404682 DOI: 10.1002/advs.202404682

Doping‐Induced Surface and Grain Boundary Effects in Ni‐Rich Layered Cathode Materials

L. Kuo, C. Roitzheim, H. Valencia, J. Mayer, S. Möller, S. Myung, M. Finsterbusch, O. Guillon, D. Fattakhova‐Rohlfing, P. Kaghazchi

Small, 2024, 20 26, e2307678 DOI: 10.1002/smll.202307678

Drum Gripping Concept for Secured Orientation-Variable Handling in Solid-State Battery Cell Assembly

D. M. Nguyen, M. Strauß, T. Scharmann, K. Dröder

N/A, 2024,  , DOI: 10.36227/techrxiv.172833203.36555819/v1

Dynamic Learning Rate Decay for Stochastic Variational Inference

M. Dinkel, G. R. Rei, W. A. Wall

arXiv (Cornell University), 2024,  , DOI: 10.48550/arxiv.2412.15745

Editors’ Choice—Alleviating the Kinetic Limitations of the Li-In Alloy Anode in All-Solid-State Batteries

S. Yanev, C. Heubner, K. Nikolowski, M. Partsch, H. Auer, A. Michaelis

Journal of The Electrochemical Society, 2024, 171 2, 020512 DOI: 10.1149/1945-7111/ad2594

Editors’ Choice—Visualizing the Impact of the Composite Cathode Microstructure and Porosity on Solid-State Battery Performance

P. Minnmann, J. Schubert, S. Kremer, R. Rekers, S. Burkhardt, R. Rueß, A. Bielefeld, F. H. Richter, J. Janek

Journal of The Electrochemical Society, 2024, 171 6, 060514 DOI: 10.1149/1945-7111/ad510e

Enabling High-Performance Hybrid Solid-State Batteries by Improving the Microstructure of Free-Standing LATP/LFP Composite Cathodes

M. Ihrig, E. Dashjav, P. Odenwald, C. Dellen, D. Grüner, J. P. Gross, T. T. H. Nguyen, Y. Lin, W. S. Scheld, C. Lee, R. Schwaiger, A. Mahmoud, J. Malzbender, O. Guillon, S. Uhlenbruck, M. Finsterbusch, F. Tietz, H. Teng, D. Fattakhova‐Rohlfing

ACS Applied Materials & Interfaces, 2024, 16 14, 17461-17473 DOI: 10.1021/acsami.3c18542

Evaluating Pressure‐dependent Discharge Behavior of Foil Versus In situ Plated Lithium Metal Anodes in Solid‐State Batteries

C. G. Haslam, J. K. Eckhardt, A. Ayyaswamy, B. S. Vishnugopi, T. Fuchs, D. W. Liao, N. P. Dasgupta, P. P. Mukherjee, J. Janek, J. Sakamoto

Advanced Energy Materials, 2024, 15 12, DOI: 10.1002/aenm.202403614

Evaluation of Oxide|Sulfide Heteroionic Interface Stability for Developing Solid-State Batteries with a Lithium–Metal Electrode: The Case of LLZO|Li6PS5Cl and LLZO|Li7P3S11

L. Merola, V. Singh, M. J. Palmer, J. K. Eckhardt, S. L. Benz, T. Fuchs, L. F. Nazar, J. Sakamoto, F. H. Richter, J. Janek

ACS Applied Materials & Interfaces, 2024, 16 40, 54847-54863 DOI: 10.1021/acsami.4c11597

Experimental correlation of anionic mass transport and lithium dendrite growth in solid-state polymer-based lithium metal batteries

J. H. Thienenkamp, P. Lennartz, M. Winter, G. Brunklaus

Cell Reports Physical Science, 2024, 5 12, 102340 DOI: 10.1016/j.xcrp.2024.102340

Exploring Layered Disorder in Lithium-Ion-Conducting Li3Y1–xInxCl6

A. Banik, B. Samanta, B. Helm, M. A. Kraft, Y. Rudel, C. Li, M. R. Hansen, B. V. Lotsch, S. Bette, W. G. Zeier

Inorganic Chemistry, 2024, 63 19, 8698-8709 DOI: 10.1021/acs.inorgchem.4c00229

External Pressure in Polymer-Based Lithium Metal Batteries: An Often-Neglected Criterion When Evaluating Cycling Performance?

P. Roering, G. M. Overhoff, K. L. Liu, M. Winter, G. Brunklaus

ACS Applied Materials & Interfaces, 2024, 16 17, 21932-21942 DOI: 10.1021/acsami.4c02095

Funktionale Beschichtung von Batteriepulvern

M. Höhn, J. P. Beaupain, E. Siebecke, M. Krug, S. Höhn

Vakuum in Forschung und Praxis, 2024, 36 3, 23-28 DOI: 10.1002/vipr.202400816

Ga-ion migration during co-sintering of heterogeneous Ta- and Ga-substituted LLZO solid-state electrolytes

W. S. Scheld, Y. Collette, C. Schwab, M. Ihrig, S. Uhlenbruck, M. Finsterbusch, D. Fattakhova‐Rohlfing

Journal of the European Ceramic Society, 2024, 45 2, 116936 DOI: 10.1016/j.jeurceramsoc.2024.116936

Grain Boundary Transport in the Argyrodite‐Type Li6PS5Br Solid Electrolyte: Influence of Misorientation and Anion Disorder on Li Ion Mobility

M. Sadowski, K. Albe

Advanced Materials Interfaces, 2024, 11 33, DOI: 10.1002/admi.202400423

Heteroionic Interfaces in Hybrid Solid-State Batteries─Current Constriction at the Interface between Different Solid Electrolytes

J. K. Eckhardt, S. Kremer, L. Merola, J. Janek

ACS Applied Materials & Interfaces, 2024, 16 14, 18222-18235 DOI: 10.1021/acsami.4c01808

Holistic view on cation interdiffusion during processing and operation of garnet all-solid-state batteries

K. Yao, W. S. Scheld, Q. Ma, Y. Zeng, S. Ganapathy, M. Ihrig, R. Ye, M. Ma, V. Kiyek, O. Guillon, M. Huijben, J. E. ten Elshof, M. Finsterbusch, D. Fattakhova‐Rohlfing

Energy storage materials, 2024, 71 , 103662 DOI: 10.1016/j.ensm.2024.103662

Imaging the microstructure of lithium and sodium metal in anode-free solid-state batteries using electron backscatter diffraction

T. Fuchs, T. Ortmann, J. Becker, C. G. Haslam, M. Ziegler, V. K. Singh, M. Rohnke, B. Mogwitz, K. Peppler, L. F. Nazar, J. Sakamoto, J. Janek

Nature Materials, 2024, 23 12, 1678-1685 DOI: 10.1038/s41563-024-02006-8

Impact of Polymer End Groups on the Formation of Solid Electrolyte Interphase at the Lithium Metal Interface: A First-Principles Calculations Study

K. Zhour, A. Heuer, D. Diddens

The Journal of Physical Chemistry C, 2024, 128 38, 15888-15898 DOI: 10.1021/acs.jpcc.4c03261

Improving the rate performance of lithium metal anodes: In-situ formation of 3D interface structures by mechanical mixing with sodium metal

M. Mann, C. Schwab, L. C. P. dos Santos, R. Spatschek, D. Fattakhova‐Rohlfing, M. Finsterbusch

Energy storage materials, 2024, 74 , 103975 DOI: 10.1016/j.ensm.2024.103975

Influence of Electrode Structuring Techniques on the Performance of All‐Solid‐State Batteries

M. Clausnitzer, T. Danner, B. Prifling, M. Neumann, V. Schmidt, A. Latz

Batteries & Supercaps, 2024, 7 4, DOI: 10.1002/batt.202300522

Influence of Post‐Synthesis Processing on the Structure, Transport, and Performance of the Solid Electrolyte Li5.5PS4.5Cl1.5 in All‐Solid‐State Batteries

O. Maus, M. Lange, F. Frankenberg, F. Stainer, V. Faka, E. Schlautmann, C. Rosenbach, A. Jodlbauer, J. Schubert, J. Janek, C. Li, P. Michalowski, M. Wilkening, A. Kwade, W. G. Zeier

Advanced Energy Materials, 2024, 15 5, DOI: 10.1002/aenm.202403291

Influence of oxygen distribution on the Li-ion conductivity in oxy-sulfide glasses – taking a closer look

R. Zimmermanns, X. Luo, A. Hansen, M. Sadowski, Q. Fu, K. Albe, S. Indris, M. Knapp, H. Ehrenberg

Dalton Transactions, 2024, 53 32, 13348-13363 DOI: 10.1039/d4dt01132e

Insights into polymer electrolyte stability and reaction pathways: A first-principle calculations study

K. Zhour, A. Heuer, D. Diddens

The Journal of Chemical Physics, 2024, 161 21, DOI: 10.1063/5.0235262

Investigating the Influence of Transition Metal Substitution in Lithium Argyrodites on Structure, Transport, and Solid-State Battery Performance

J. Härtel, A. Banik, M. Y. Ali, B. Helm, K. Strotmann, V. Faka, O. Maus, C. Li, H. Wiggers, W. G. Zeier

Chemistry of Materials, 2024, 36 21, 10731-10745 DOI: 10.1021/acs.chemmater.4c02281

In–Li Counter Electrodes in Solid‐State Batteries – A Comparative Approach on Kinetics, Microstructure, and Chemomechanics

C. D. Alt, S. Keuntje, I. Schneider, J. A. Westphal, P. Minnmann, J. K. Eckhardt, K. Peppler, J. Janek

Advanced Energy Materials, 2024, 15 12, DOI: 10.1002/aenm.202404055

Lithiated polymer coating for interface stabilization in Li6PS5Cl-based solid-state batteries with high-nickel NCM

B. Shi, F. Weber, Y. Yusim, T. Demuth, K. Vettori, A. Münchinger, G. Titvinidze, K. Volz, A. Henß, R. Berger, F. H. Richter

Journal of Materials Chemistry A, 2024, 13 4, 2600-2614 DOI: 10.1039/d4ta07265k

Lithium All‐Solid‐State Batteries Fabricated at Room Temperature by the Powder Aerosol Deposition Method with Garnet‐Type Electrolyte and Graded Composite Cathode

L. Hennerici, P. Ficht, M. Schamel, U. Mansfeld, M. Linz, D. Paulus, J. Kita, M. A. Danzer, R. Moos

Advanced Materials Technologies, 2024, 10 3, DOI: 10.1002/admt.202400745

Microstructure, Charge Transport and Interfaces in All-Solid-State Batteries

F. Hartmann, J. Janek

ECS Meeting Abstracts, 2024, MA2024-02 8, 1188 DOI: 10.1149/ma2024-0281188mtgabs

My cell is better than yours

N. M. Vargas‐Barbosa

Nature Nanotechnology, 2024, 19 4, 419-420 DOI: 10.1038/s41565-024-01607-3

Operando Photoelectron Spectroscopy Analysis of Li 6 PS 5 Cl Electrochemical Decomposition Reactions in Solid-State Batteries

B. Aktekin, E. Kataev, L. M. Riegger, R. Garcia‐Diez, Z. Chalkley, J. Becker, R. G. Wilks, A. Henß, M. Bär, J. Janek

ACS Energy Letters, 2024, 9 7, 3492-3500 DOI: 10.1021/acsenergylett.4c01072

Protective Nanosheet Coatings for Thiophosphate‐Based All‐Solid‐State Batteries

L. Karger, B. N. Nunes, Y. Yusim, A. Mazilkin, R. Zhang, W. Zhao, A. Henß, A. Kondrakov, J. Janek, T. Brezesinski

Advanced Materials Interfaces, 2024, 11 14, DOI: 10.1002/admi.202301067

Quantifying multiphase SEI growth in sulfide solid electrolytes

C. D. Alt, N. U. Müller, L. M. Riegger, B. Aktekin, P. Minnmann, K. Peppler, J. Janek

Joule, 2024, 8 10, 2755-2776 DOI: 10.1016/j.joule.2024.07.006

Reducing the Defect Formation Energy by Aliovalent Sn(+IV) and Isovalent P(+V) Substitution in Li3SbS4 Promotes Li+ Transport

B. Helm, K. Strotmann, T. Böger, B. Samanta, A. Banik, M. Lange, Y. Li, C. Li, M. R. Hansen, P. Canepa, W. G. Zeier

ACS Applied Energy Materials, 2024, 7 5, 1735-1747 DOI: 10.1021/acsaem.3c02652

Reducing the environmental footprint of solid-electrolytes - a green synthesis route for LATP

M. Rosen, P. Hecker, M. Mann, Q. Ma, J. P. Gross, R. Schwaiger, O. Guillon, D. Fattakhova‐Rohlfing, M. Finsterbusch

Green Chemistry, 2024, 26 5, 2712-2720 DOI: 10.1039/d3gc03293k

Sodium Filling in Superadamantoide Na1.36(Si0.86Ga0.14)2As2.98 and the Mixed Valent Arsenidosilicate-Silicide Li1.5Ga0.9Si3.1As4

M. Schöneich, L. G. Balzat, B. V. Lotsch, D. Johrendt

Inorganics, 2024, 12 6, 166 DOI: 10.3390/inorganics12060166

Solving Bayesian inverse problems with expensive likelihoods using constrained Gaussian processes and active learning

M. Dinkel, C. M. Geitner, G. R. Rei, J. Nitzler, W. A. Wall

Inverse Problems, 2024, 40 9, 095008 DOI: 10.1088/1361-6420/ad5eb4

Spray-Flame Synthesis of NASICON-Type Rhombohedral (α) Li1+xYxZr2−x(PO4)3 [x = 0–0.2] Solid Electrolytes

M. Y. Ali, T. Chen, H. Orthner, H. Wiggers

Nanomaterials, 2024, 14 15, 1278 DOI: 10.3390/nano14151278

Synergistic Enhancement of Mechanical and Electrochemical Properties in Grafted Polymer/Oxide Hybrid Electrolytes

F. Scharf, A. Krude, P. Lennartz, M. Clausnitzer, G. Shukla, A. Buchheit, F. Kempe, D. Diddens, P. Glomb, M. M. Mitchell, T. Danner, A. Heuer, A. Latz, M. Winter, G. Brunklaus

Small, 2024, 20 47, e2404537 DOI: 10.1002/smll.202404537

Ternary Solid Polymer Electrolytes at the Electrochemical Interface: A Computational Study

A. Rivera-Pousa, J. M. Otero-Mato, H. Montes‐Campos, T. Méndez‐Morales, D. Diddens, A. Heuer, L. M. Varela

Macromolecules, 2024, 57 9, 3921-3936 DOI: 10.1021/acs.macromol.3c02669

The Formation of Residual Lithium Compounds on Ni‐Rich NCM Oxides: Their Impact on the Electrochemical Performance of Sulfide‐Based ASSBs

B. Aktekin, A. E. Sedykh, K. Müller‐Buschbaum, A. Henß, J. Janek

Advanced Functional Materials, 2024, 34 21, DOI: 10.1002/adfm.202313252

The Li battery digital twin – Combining 4D modelling, electro-chemistry, neutron, and ion-beam techniques

S. Möller, C. Schwab, S. Seidlmayer, M. Clausnitzer, M. Rosen, J. Hormann, M. Mann, A. Cannavò, G. Ceccio, J. Vacı́k, K. Mouzakka, T. Danner, A. Latz, R. Gilles, M. Finsterbusch

Journal of Power Sources, 2024, 610 , 234681 DOI: 10.1016/j.jpowsour.2024.234681

The impact of lithium carbonate on tape cast LLZO battery separators: A balanced interplay between lithium loss and relithiation

K. Touidjine, M. Finsterbusch-Rosen, V. Kiyek, S. Ganapathy, M. Finsterbusch, O. Guillon, M. Huijben, E. M. Kelder, M. Wagemaker, D. Fattakhova‐Rohlfing

Energy storage materials, 2024, 71 , 103487 DOI: 10.1016/j.ensm.2024.103487

“Depo-All-Around”: A Novel FIB-Based TEM Specimen Preparation Technique For Solid State Battery Composites And Other Loosely Bound Samples

T. Demuth, T. Fuchs, A. Beyer, J. Janek, K. Volz

Ultramicroscopy, 2024, 257 , 113904 DOI: 10.1016/j.ultramic.2023.113904

A Conservative And Efficient Model For Grain Boundaries Of Solid Electrolytes In A Continuum Model For Solid-State Batteries

S. Sinzig, C. P. Schmidt, W. A. Wall

Journal of The Electrochemical Society, 2024, 171 4, 040505 DOI: 10.1149/1945-7111/ad36e4

Benchmarking Of Coatings For Cathode Active Materials In Solid-State Batteries Using Surface Analysis And Reference Electrodes

J. Hertle, F. Walther, T. Lombardo, C. Kern, B. Pavlovic, B. Mogwitz, X. Wu, H. Schneider, M. Rohnke, J. Janek

ACS Applied Materials & Interfaces, 2024, 16 7, 9400-9413 DOI: 10.1021/acsami.3c15723

Blacklight Sintering Of Garnet-Based Composite Cathodes

W. S. Scheld, J.N. Ebert, M. Scherer, L. Fulanovic, L. Porz, C. Dellen, M. Ihrig, S. Uhlenbruck, M. Finsterbusch, O. Guillon, D. Fattakhova-Rohlfing, W. Rheinheimer

Journal of the European Ceramic Society, 2024, 44 5, 3039-3048 DOI: 10.1016/j.jeurceramsoc.2023.12.040

Chemo-Mechanical Failure Mechanisms Of The Silicon Anode In Solid-State Batteries

H. Huo, M. Jiang, Y. Bai, S. Ahmed, K. Volz, H. Hartmann, A. Henss, C. V. Singh, D. Raabe, J. Janek

Nature Materials, 2024, 23 4, 543-551 DOI: 10.1038/s41563-023-01792-x

Degradation Of Styrene-Poly(Ethylene Oxide)-Based Block Copolymer Electrolytes At The Na And K Negative Electrode Studied By Microcalorimetry And Impedance Spectroscopy

S. Xing, A. Khudyshkina, U.-C. Rauska, A. J. Butzelaar, D. Voll, P. Theato, J. Tübke, F. Jeschull

Journal of The Electrochemical Society, 2024, 171 4, 040516 DOI: 10.1149/1945-7111/ad3b72

Doping-Induced Surface And Grain Boundary Effects In Ni-Rich Layered Cathode Materials

L.-Y. Kuo, C. Roitzheim, H. Valencia, J. Mayer, S. Möller, S.-T. Myung, M. Finsterbusch, O. Guillon, D. Fattakhova-Rohlfing, P. Kaghazchi

Small, 2024,  , 2307678 DOI: 10.1002/smll.202307678

Editors’ Choice—Alleviating The Kinetic Limitations Of The Li-In Alloy Anode In All-Solid-State Batteries

S. Yanev, C. Heubner, K. Nikolowski, M. Partsch, H. Auer, A. Michaelis

Journal of The Electrochemical Society, 2024, 171 2, 020512 DOI: 10.1149/1945-7111/ad2594

Enabling High-Performance Hybrid Solid-State Batteries By Improving The Microstructure Of Free-Standing LATP/LFP Composite Cathodes

M. Ihrig, E. Dashjav, P. Odenwald, C. Dellen, D. Grüner, J. P. Gross, T. T. H. Nguyen, Y.-H. Lin, W. S. Scheld, C. Lee, R. Schwaiger, A. Mahmoud, J. Malzbender, O. Guillon, S. Uhlenbruck, M. Finsterbusch, F. Tietz, H. Teng, D. Fattakhova-Rohlfing

ACS Applied Materials & Interfaces, 2024, 16 14, 17461-17473 DOI: 10.1021/acsami.3c18542

Heteroionic Interfaces In Hybrid Solid-State Batteries─Current Constriction At The Interface Between Different Solid Electrolytes

J. K. Eckhardt, S. Kremer, L. Merola, J. Janek

ACS Applied Materials & Interfaces, 2024, 16 14, 18222-18235 DOI: 10.1021/acsami.4c01808

Impact Of Degradation Mechanisms At The Cathode/Electrolyte Interface Of Garnet-Based All-Solid-State Batteries

M. Clausnitzer, M. Ihrig, L. Cressa, S. Hein, M. Finsterbusch, S. Eswara, L.-Y. Kuo, T. Danner, P. Kaghazchi, D. Fattakhova-Rohlfing, O. Guillon, A. Latz

Energy Storage Materials, 2024, 67 , 103262 DOI: 10.1016/j.ensm.2024.103262

Influence Of Electrode Structuring Techniques On The Performance Of All-Solid-State Batteries

M. Clausnitzer, T. Danner, B. Prifling, M. Neumann, V. Schmidt, A. Latz

Batteries & Supercaps, 2024, 7 4, e202300522 DOI: 10.1002/batt.202300522

Investigation Of The Stability Of The Poly(Ethylene Oxide)|LiNi_1-X-YCo_xMn_yO₂ Interface In Solid-State Batteries

Y. Yusim, D. F. Hunstock, A. Mayer, D. Bresser, S. Passerini, J. Janek, A. Henss

Advanced Materials Interfaces, 2024, 11 3, 2300532 DOI: 10.1002/admi.202300532

Metal Electrodes For Next-Generation Rechargeable Batteries

G. Brunklaus, P. Lennartz, M. Winter

Nature Reviews Electrical Engineering, 2024, 1 2, 79-92 DOI: 10.1038/s44287-023-00006-5

Modelling Atomic And Nanoscale Structure In The Silicon–Oxygen System Through Active Machine Learning

L. C. Erhard, J. Rohrer, K. Albe, V. L. Deringer

Nature Communications, 2024, 15 1, 1927 DOI: 10.1038/s41467-024-45840-9

My Cell Is Better Than Yours

N. M. Vargas-Barbosa

Nature Nanotechnology, 2024, 19 4, 419-420 DOI: 10.1038/s41565-024-01607-3

Protective Nanosheet Coatings For Thiophosphate-Based All-Solid-State Batteries

L. Karger, B. N. Nunes, Y. Yusim, A. Mazilkin, R. Zhang, W. Zhao, A. Henss, A. Kondrakov, J. Janek, T. Brezesinski

Advanced Materials Interfaces, 2024, 11 14, 2301067 DOI: 10.1002/admi.202301067

Recycling Of Solid-State Batteries

M. Ahuis, S. Doose, D. Vogt, P. Michalowski, S. Zellmer, A. Kwade

Nature Energy, 2024, 9 4, 373-385 DOI: 10.1038/s41560-024-01463-4

Reducing The Environmental Footprint Of Solid-Electrolytes - A Green Synthesis Route For LATP

M. Rosen, P. Hecker, M. Mann, Q. Ma, J. P. Peter Gross, R. Schwaiger, O. Guillon, D. Fattakhova-Rohlfing, M. Finsterbusch

Green Chemistry, 2024, 26 5, 2712-2720 DOI: 10.1039/D3GC03293K

Revealing The Deposition Mechanism Of The Powder Aerosol Deposition Method Using Ceramic Oxide Core–Shell Particles

M. Linz, F. Bühner, D. Paulus, L. Hennerici, Y. Guo, V. Mereacre, U. Mansfeld, M. Seipenbusch, J. Kita, R. Moos

Advanced Materials, 2024, 36 7, 2308294 DOI: 10.1002/adma.202308294

State Of Charge-Dependent Impedance Spectroscopy As A Helpful Tool To Identify Reasons For Fast Capacity Fading In All-Solid-State Batteries

M. Wiche, Y. Yusim, K. Vettori, R Ruess, A Henss, M. T. Elm

ACS Applied Materials & Interfaces, 2024, 16 3, 3253-3259 DOI: 10.1021/acsami.3c13160

Towards Automatic Feature Extraction And Sample Generation Of Grain Structure By Variational Autoencoder

Y. Ji, A. Koeppe, P. Altschuh, D. Rajagopal, Y. Zhao, W. Chen, Y. Zhang, Y. Zheng, B. Nestler

Computational Materials Science, 2024, 232, 112628 DOI: 10.1016/j.commatsci.2023.112628

2023

A Layered Hybrid Oxide–Sulfide All-Solid-State Battery With Lithium Metal Anode

J. Hüttl, N. Zapp, S. Tanikawa, K. Nikolowski, A. Michaelis, H. Auer

Batteries, 2023, 9 10, 507 DOI: 10.3390/batteries9100507

An Efficient Approach To Include Transport Effects In Thin Coating Layers In Electrochemo-Mechanical Models For All-Solid-State Batteries

S. Sinzig, C. P. Schmidt, W. A. Wall

Journal of The Electrochemical Society, 2023, 170 10, 100532 DOI: 10.1149/1945-7111/ad0264

Combining Nitridoborates, Nitrides And Hydrides—Synthesis And Characterization Of The Multianionic Sr₆N[BN₂]₂H₃

S. L. Wandelt, A. Mutschke, D. Khalyavin, R. Calaminus, J. Steinadler, B. V. Lotsch, W. Schnick

Angewandte Chemie, 2023, 135 50, e202313564 DOI: 10.1002/ange.202313564

Co-Sintering Of Li_1.3Al_0.3Ti_1.7(PO₄)₃ And LiFePO₄ In Tape-Casted Composite Cathodes For Oxide Solid-State Batteries

J. Beaupain, K. Waetzig, H. Auer, N. Zapp, K. Nikolowski, M. Partsch, M. Kusnezoff, A. Michaelis

Batteries, 2023, 9 11, 543 DOI: 10.3390/batteries9110543

Enabling Metal Substrates For Garnet-Based Composite Cathodes By Laser Sintering

W. S. Scheld, L. C. Hoff, C. Vedder, J. Stollenwerk, D. Grüner, M. Rosen, S. Lobe, M. Ihrig, A.-R. Seok, M. Finsterbusch, S. Uhlenbruck, O. Guillon, D. Fattakhova–Rohlfing

Applied Energy, 2023, 345 , 121335 DOI: 10.1016/j.apenergy.2023.121335

Finding Order In Disorder: The Highly Disordered Lithium Oxonitridophosphate Double Salt Li_8+XP₃O_10−XN_1+X (X=1.4(5))

S. Schneider, S. T. Kreiner, L. G. Balzat, B. V. Lotsch, W. Schnick

Chemistry – A European Journal, 2023, 29 55, e202301986 DOI: 10.1002/chem.202301986

Functionalized Thiophosphate And Oxidic Filler Particles For Hybrid Solid Electrolytes

L. Helmers, F. Frankenberg, J. Brokmann, C. Burmeister, A. Buchheit, A. Kwade, P. Michalowski

ChemElectroChem, 2023, 10 21, e202300310 DOI: 10.1002/celc.202300310

Guidelines For Impedance Analysis Of Parent Metal Anodes In Solid-State Batteries And The Role Of Current Constriction At Interface Voids, Heterogeneities, And SEI

J. K. Eckhardt, T. Fuchs, S. Burkhardt, P. J. Klar, J. Janek, C. Heiliger

Advanced Materials Interfaces, 2023, 10 8, 2202354 DOI: 10.1002/admi.202202354

Impact Of Polymer End Groups On The Formation Of Solid Electrolyte Interphase At The Lithium Metal Interface: A First-Principle Calculations Study

K. Zhour, A. Heuer, D. Diddens

2023,  , DOI: 10.2139/ssrn.4591491

Impact Of The Solid Electrolyte Particle Size Distribution In Sulfide-Based Solid-State Battery Composites

E. Schlautmann, A. Weiß, O. Maus, L. Ketter, M. Rana, S. Puls, V. Nickel, C. Gabbey, C. Hartnig, A. Bielefeld, W. G. Zeier

Advanced Energy Materials, 2023, 13 41, 2302309 DOI: 10.1002/aenm.202302309

Improved Route To Linear Triblock Copolymers By Coupling With Glycidyl Ether-Activated Poly(Ethylene Oxide) Chains

D. T. Krause, S. Krämer, V. Siozios, A. J. Butzelaar, M. Dulle, B. Förster, P. Theato, J. Mayer, M. Winter, S. Förster, H.-D. Wiemhöfer, M. Grünebaum

Polymers, 2023, 15 9, 2128 DOI: 10.3390/polym15092128

Li_3–XZr_x(Ho/Lu)_1–XCl Solid Electrolytes Enable Ultrahigh-Loading Solid-State Batteries With A Prelithiated Si Anode

L. Zhou, T. Zuo, C. Li, Q. Zhang, J. Janek, L. F. Nazar

ACS Energy Letters, 2023, 8 7, 3102-3111 DOI: 10.1021/acsenergylett.3c00763

Microstructural Parameters Governing The Mechanical Stress And Conductivity Of All-Solid-State Lithium-Ion-Battery Cathodes

F. Al-Jaljouli, R. Mücke, P. Kaghazchi, Y. J. Sohn, M. Finsterbusch, D. Fattakhova-Rohlfing, O. Guillon

Journal of Energy Storage, 2023, 68 , 107784 DOI: 10.1016/j.est.2023.107784

Modelling Electro-Chemically Induced Stresses In All-Solid-State Batteries: Screening Electrolyte And Cathode Materials In Composite Cathodes

R. Mücke, N. Yaqoob, M. Finsterbusch, F. Al-Jaljouli, P. Kaghazchi, D. Fattakhova-Rohlfing, O. Guillon

Journal of Materials Chemistry A, 2023, 11 35, 18801-18810 DOI: 10.1039/D3TA01729J

Nanocrystalline Cellulose Reinforced Poly(Ethylene Oxide) Electrolytes For Lithium-Metal Batteries With Excellent Cycling Stability

G.-T. Kim, C. Antonelli, C. Iojoiu, M. Löffler, D. Bresser, Y. Molméret, J.-Y. Sanchez, S. Passerini

Frontiers in Energy Research, 2023, 11 , DOI: 10.3389/fenrg.2023.1325612

Optimizing The Composite Cathode Microstructure In All-Solid-State Batteries By Structure-Resolved Simulations

M. Clausnitzer, R. Mücke, F. Al-Jaljouli, S. Hein, M. Finsterbusch, T. Danner, D. Fattakhova-Rohlfing, O. Guillon, A. Latz

Batteries & Supercaps, 2023, 6 11, e202300167 DOI: 10.1002/batt.202300167

Pressure Dependence Of Ionic Conductivity In Site Disordered Lithium Superionic Argyrodite Li₆PS₅Br

V. Faka, M. T. Agne, P. Till, T. Bernges, M. Sadowski, A. Gautam, K. Albe, W. G. Zeier

Energy Advances, 2023, 2 11, 1915-1925 DOI: 10.1039/D3YA00424D

Solid Electrolyte Cracking Due To Lithium Filament Growth And Concept Of Mechanical Reinforcement – An Operando Study

J. Duan, T. Fuchs, B. Mogwitz, P. Minnmann, T. Zuo, A. Henss, J. Janek

Materials Today, 2023, 70 , 33-43 DOI: 10.1016/j.mattod.2023.10.003

The Riddle Of Dark LLZO: Cobalt Diffusion In Garnet Separators Of Solid-State Lithium Batteries

W. S. Scheld, K. Kim, C. Schwab, A. C. Moy, S.-K. Jiang, M. Mann, C. Dellen, Y. J. Sohn, S. Lobe, M. Ihrig, M. G. Danner, C.-Y. Chang, S. Uhlenbruck, E. D. Wachsman, B. J. Hwang, J. Sakamoto, L. F. Wan, B. C. Wood, M. Finsterbusch, D. Fattakhova-Rohlfing

Advanced Functional Materials, 2023, 33 43, 2302939 DOI: 10.1002/adfm.202302939

Understanding Lithium-Ion Transport In Selenophosphate-Based Lithium Argyrodites And Their Limitations In Solid-State Batteries

J. Hartel, A. Banik, J. M. Gerdes, B. Wankmiller, B. Helm, C. Li, M. A. Kraft, M. R. Hansen, W. G. Zeier

Chemistry of Materials, 2023, 35 12, 4798-4809 DOI: 10.1021/acs.chemmater.3c00658

An Efficient Approach to Include Transport Effects in Thin Coating Layers in Electrochemo-Mechanical Models for All-Solid-State Batteries

S. Sinzig, C. P. Schmidt, W. A. Wall

Journal of The Electrochemical Society, 2023, 170, 100532 DOI: 10.1149/1945-7111/ad0264

Probing The Ni(OH)₂ Precursor For LiNiO₂ At The Atomic Scale: Insights Into The Origin Of Structural Defect In A Layered Cathode Active Material

A. Pokle, D. Weber, M. Bianchini, J. Janek, K. Volz

Small, 2023, 19 (4), 2205508 DOI: 10.1002/smll.202205508

Polypropylene Carbonate-Based Electrolytes As Model For A Different Approach Towards Improved Ion Transport Properties For Novel Electrolytes

A. I. Gerlitz, D. Diddens, M. Grünebaum, A. Heuer, M. Winter, H. Wiemhöfer

Physical Chemistry Chemical Physics, 2023, 25 (6), 4810-4823 DOI: 10.1039/D2CP03756D

Solid-State Batteries: From ‘All-Solid’ To ‘Almost-Solid’

H. Huo, J. Janek

National Science Review, 2023, 10 (6), nwad098 DOI: 10.1093/nsr/nwad098

Challenges In Speeding Up Solid-State Battery Development

J. Janek, W. G. Zeier

Nature Energy, 2023, 8 (3), 230-240 DOI: 10.1038/s41560-023-01208-9

Understanding The Evolution Of Lithium Dendrites At Li_6.25Al_0.25La₃Zr₂O₁₂ Grain Boundaries Via Operando Microscopy Techniques

C. Zhu, T. Fuchs, S. A. L. Weber, F. H. Richter, G. Glasser, F. Weber, H. Butt, J. Janek, R. Berger

Nature Communications, 2023, 14 (1), 1300 DOI: 10.1038/s41467-023-36792-7

SEI Growth On Lithium Metal Anodes In Solid-State Batteries Quantified With Coulometric Titration Time Analysis

B. Aktekin, L. M. Riegger, S. Otto, T. Fuchs, A. Henss, J. Janek

Nature Communications, 2023, 14 (1), 6946 DOI: 10.1038/s41467-023-42512-y

Acid Leaching Of Al- And Ta-Substituted Li₇La₃Zr₂O₁₂ (LLZO) Solid Electrolyte

K. Schneider, V. Kiyek, M. Finsterbusch, B. Yagmurlu, D. Goldmann

Metals, 2023, 13 (5), 834 DOI: 10.3390/met13050834

Origin Of The Lithium Metal Anode Instability In Solid-State Batteries During Discharge

D. K. Singh, T. Fuchs, C. Krempaszky, P. Schweitzer, C. Lerch, F. H. Richter, J. Janek

Matter, 2023, 6 (5), 1463-1483 DOI: 10.1016/j.matt.2023.02.008

Influence Of The Sintering Temperature On LLZO-NCM Cathode Composites For Solid-State Batteries Studied By Transmission Electron Microscopy

T. Demuth, T. Fuchs, F. Walther, A. Pokle, S. Ahmed, M. Malaki, A. Beyer, J. Janek, K. Volz

Matter, 2023, 6 (7), 2324-2339 DOI: 10.1016/j.matt.2023.04.022

Investigation Of The Structure And Ionic Conductivity Of A Li₃InCl₆ Modified By Dry Room Annealing For Solid-State Li-Ion Battery Applications

P. Molaiyan, S. E. Mailhiot, K. Voges, A. M. Kantola, T. Hu, P. Michalowski, A. Kwade, V. Telkki, U. Lassi

Materials & Design, 2023, 227, 111690 DOI: 10.1016/j.matdes.2023.111690

Bisphenol-Derived Single-Ion Conducting Multiblock Copolymers As Lithium Battery Electrolytes: Impact Of The Bisphenol Building Block

A. Mayer, A. Mariani, X. Dong, G. Vansse, P. Theato, C. Iojoiu, S. Passerini, D. Bresser

Macromolecules, 2023, 56 (6), 2505-2514 DOI: 10.1021/acs.macromol.2c02404

Towards Economic Processing Of High Performance Garnets – Case Study On Zero Li Excess Ga-Substituted LLZO

C. Schwab, G. Häuschen, M. Mann, C. Roitzheim, O. Guillon, D. Fattakhova-Rohlfing, M. Finsterbusch

Journal of Materials Chemistry A, 2023, 11 (11), 5670-5680 DOI: 10.1039/D2TA09250F

Stepwise Optimization Of Single-Ion Conducting Polymer Electrolytes For High-Performance Lithium-Metal Batteries

X. Dong, Z. Chen, X. Gao, A. Mayer, H. Liang, S. Passerini, D. Bresser

Journal of Energy Chemistry, 2023, 80, 174-181 DOI: 10.1016/j.jechem.2023.01.044

Single-Crystalline LiNiO₂ As High-Capacity Cathode Active Material For Solid-State Lithium-Ion Batteries

R. Rueß, D. Gomboso, M. Ulherr, E. Trevisanello, Y. Ma, A. Kondrakov, T. Brezesinski, J. Janek

Journal of The Electrochemical Society, 2023, 170 (2), 20533 DOI: 10.1149/1945-7111/acbc4f

Miniaturization Of Reference Electrodes For Solid-State Lithium-Ion Batteries

J. Hertle, F. Walther, B. Mogwitz, S. Schröder, X. Wu, F. H. Richter, J. Janek

Journal of The Electrochemical Society, 2023, 170 (4), 40519 DOI: 10.1149/1945-7111/accb6f

Oxide Ceramic Electrolytes For All-Solid-State Lithium Batteries – Cost-Cutting Cell Design And Environmental Impact

A. Schreiber, M. Rosen, K. Waetzig, K. Nikolowski, N. Schiffmann, H. Wiggers, M. Küpers, D. Fattakhova-Rohlfing, W. Kuckshinrichs, O. Guillon, M. Finsterbusch

Green Chemistry, 2023, 25 (1), 399-414 DOI: 10.1039/D2GC03368B

Synthesis And Application Of An Aromatic Sulfonate Sodium Salt For Aqueous Sodium-Ion Battery Electrolytes

X. Dong, X. Liu, J. Han, Z. Chen, H. Zhang, S. Passerini, D. Bresser

Energy Technology, 2023, 11 (1), 2201045 DOI: 10.1002/ente.202201045

Nanostructured Block Copolymer Single-Ion Conductors For Low-Temperature, High-Voltage And Fast Charging Lithium-Metal Batteries

J. Shi, H. Nguyen, Z. Chen, R. Wang, D. Steinle, L. Barnsley, J. Li, H. Frielinghaus, D. Bresser, C. Iojoiu, E. Paillard

Energy Materials, 2023, 3 (4), 30036  DOI: 10.20517/energymater.2023.27

From Lithium To Potassium: Comparison Of Cations In Poly(Ethylene Oxide)-Based Block Copolymer Electrolytes For Solid-State Alkali Metal Batteries

A. D. Khudyshkina, A. J. Butzelaar, Y. Guo, M. Hoffmann, T. Bergfeldt, M. Schaller, S. Indris, M. Wilhelm, P. Théato, F. Jeschull

Electrochimica Acta, 2023, 454, 142421 DOI: 10.1016/j.electacta.2023.142421

A Three-Dimensional Finite Element Formulation Coupling Electrochemistry And Solid Mechanics On Resolved Microstructures Of All-Solid-State Lithium-Ion Batteries

C. P. Schmidt, S. Sinzig, V. Gravemeier, W. A. Wall

Computer Methods in Applied Mechanics and Engineering, 2023, 417, 116468 DOI: 10.1016/j.cma.2023.116468

Recycling Of All-Solid-State Li-Ion Batteries: A Case Study Of The Separation Of Individual Components Within A System Composed Of LTO, LLZTO And NMC

A. I. Waidha, A. Salihovic, M. Jacob, V. Vanita, B. Aktekin, K. Brix, K. Wissel, R. Kautenburger, J. Janek, W. Ensinger, O. Clemens

ChemSusChem, 2023, 16 (13), e202202361 DOI: 10.1002/cssc.202202361

Evolution Of The Interphase Between Argyrodite-Based Solid Electrolytes And The Lithium Metal Anode─The Kinetics Of Solid Electrolyte Interphase Growth

L. M. Riegger, S. Mittelsdorf, T. Fuchs, R. Rueß, F. H. Richter, J. Janek

Chemistry of Materials, 2023, 35 (13), 5091-5099 DOI: 10.1021/acs.chemmater.3c00676

Impact Of Ni–Mn–Co–Al-Based Cathode Material Composition On The Sintering With Garnet Solid Electrolytes For All-Solid-State Batteries

A. Bauer, C. Roitzheim, S. Lobe, Y. J. Sohn, D. Sebold, W. S. Scheld, M. Finsterbusch, O. Guillon, D. Fattakhova-Rohlfing, S. Uhlenbruck

Chemistry of Materials, 2023, 35 (21), 8958-8968 DOI: 10.1021/acs.chemmater.3c01573

Ultrathin Single-Ion Conducting Polymer Enabling A Stable Li|Li_1.3Al_0.3Ti_1.7(PO₄)₃ Interface

Z. Chen, H. Liang, Z. Lyu, N. Paul, G. Ceccio, R. Gilles, M. Zarrabeitia, A. Innocenti, M. Jasarevic, G. Kim, S. Passerini, D. Bresser

Chemical Engineering Journal, 2023, 467, 143530 DOI: 10.1016/j.cej.2023.143530

A Finite Element Formulation To Three-Dimensionally Resolve Space-Charge Layers In Solid Electrolytes

S. Sinzig, T. Hollweck, C. P. Schmidt, W. A. Wall

Journal of The Electrochemical Society, 2023, 170, 040513, DOI: 10.1149/1945-7111/acc692

Modelling Atomic And Nanoscale Structure In The Silicon-Oxygen System Through Active Machine Learning

L. C. Erhard, J. Rohrer, K. Albe, V. L. Deringer

arXiv, 2023, arXiv:2309.03587, DOI: 10.48550/arXiv.2309.03587

Evaluation And Improvement Of The Stability Of Poly(Ethylene Oxide)-Based Solid-State Batteries With High-Voltage Cathodes

Y. Yusim, E. Trevisanello, R. Ruess, F. H. Richter, A. Mayer, D. Bresser, S. Passerini, J. Janek, A. Henss

Angewandte Chemie International Edition, 2023, 62 (12), e202218316 DOI: 10.1002/anie.202218316

Impact Of The Chlorination Of Lithium Argyrodites On The Electrolyte/Cathode Interface In Solid-State Batteries

T. Zuo, F. Walther, J. H. Teo, R. Rueß, Y. Wang, M. Rohnke, D. Schröder, L. F. Nazar, J. Janek

Angewandte Chemie International Edition, 2023, 62 (7), e202213228 DOI: 10.1002/anie.202213228

Interface Design Enabling Stable Polymer/Thiophosphate Electrolyte Separators For Dendrite-Free Lithium Metal Batteries

H. Huo, M. Jiang, B. Mogwitz, J. Sann, Y. Yusim, T. Zuo, Y. Moryson, P. Minnmann, F. H. Richter, C. Veer Singh, J. Janek

Angewandte Chemie International Edition, 2023, 62 (14), e202218044 DOI: 10.1002/anie.202218044

Evaluierung Und Verbesserung Der Stabilität Von Poly(Ethylenoxid)-Basierten Festkörperbatterien Mit Hochvoltkathoden

Y. Yusim, E. Trevisanello, R. Ruess, F. H. Richter, A. Mayer, D. Bresser, S. Passerini, J. Janek, A. Henss

Angewandte Chemie, 2023, 135 (12), e202218316 DOI: 10.1002/ange.202218316

Non-Linear Kinetics Of The Lithium Metal Anode On Li₆PS₅Cl At High Current Density: Dendrite Growth And The Role Of Lithium Microstructure On Creep

D. K. Singh, T. Fuchs, C. Krempaszky, B. Mogwitz, J. Janek

Advanced Science, 2023, 10 (22), 2302521 DOI: 10.1002/advs.202302521

Typology Of Battery Cells – From Liquid To Solid Electrolytes

S. Sen, F. H. Richter

Advanced Science, 2023, 2303985 DOI: 10.1002/advs.202303985

Effective Mechanochemical Synthesis Of Sulfide Solid Electrolyte Li₃PS₄ In A High Energy Ball Mill By Process Investigation

M. Hofer, M. Grube, C. F. Burmeister, P. Michalowski, S. Zellmer, A. Kwade

Advanced Powder Technology, 2023, 34 (6), 104004 DOI: 10.1016/j.apt.2023.104004

Coating Versus Doping: Understanding The Enhanced Performance Of High-Voltage Batteries By The Coating Of Spinel LiNi_0.5Mn_1.5O₄ With Li_0.35La_0.55TiO₃

V. Mereacre, P. Stüble, V. Trouillet, S. Ahmed, K. Volz, J. R. Binder

Advanced Materials Interfaces, 2023, 10 (2), 2201324 DOI: 10.1002/admi.202201324

Guidelines For Impedance Analysis Of Parent Metal Anodes In Solid-State Batteries And The Role Of Current Constriction At Interface Voids, Heterogeneities, And SEI

J. K. Eckhardt, T. Fuchs, S. Burkhardt, P. J. Klar, J. Janek, C. Heiliger

Advanced Materials Interfaces, 2023, 10 (8), 2202354 DOI: 10.1002/admi.202202354

Probing The Interface Evolution In Co-Sintered All-Phosphate Cathode-Solid Electrolyte Composites

M. Malaki, J. Haust, J. P. Beaupain, H. Auer, A. Beyer, K. Wätzig, M. Kusnezoff, K. Volz

Advanced Materials Interfaces, 2023, 2300513 DOI: 10.1002/admi.202300513

Bridging The Gap: Electrode Microstructure And Interphase Characterization By Combining ToF-SIMS And Machine Learning

T. Lombardo, C. Kern, J. Sann, M. Rohnke, J. Janek

Advanced Materials Interfaces, 2023, 2300640 DOI: 10.1002/admi.202300640

Revealing The Deposition Mechanism Of The Powder Aerosol Deposition Method Using Ceramic Oxide Core-Shell Particles

M. Linz, F. Bühner, D. Paulus, L. Hennerici, Y. Guo, V. Mereacre, U. Mansfeld, M. Seipenbusch, J. Kita, R. Moos

Advanced Materials, 2023, 2308294 DOI: 10.1002/adma.202308294

Overcoming Anode Instability In Solid-State Batteries Through Control Of The Lithium Metal Microstructure

D. K. Singh, T. Fuchs, C. Krempaszky, B. Mogwitz, S. Burkhardt, F. H. Richter, J. Janek

Advanced Functional Materials, 2023, 33 (1), 2211067 DOI: 10.1002/adfm.202211067

Towards All-Solid-State Polymer Batteries: Going Beyond PEO With Hybrid Concepts

Y. Chen, P. Lennartz, K. L. Liu, Y. Hsieh, F. Scharf, R. Guerdelli, A. Buchheit, M. Grünebaum, F. Kempe, M. Winter, G. Brunklaus

Advanced Functional Materials, 2023, 33 (32), 2300501 DOI: 10.1002/adfm.202300501

Benchmarking And Critical Design Considerations Of Zero-Excess Li-Metal Batteries

O. Lohrberg, K. Voigt, S. Maletti, H. Auer, K. Nikolowski, C. Heubner, A. Michaelis

Advanced Functional Materials, 2023, 33 (24), 2214891 DOI: 10.1002/adfm.202214891

Visualizing The Chemical Incompatibility Of Halide And Sulfide-Based Electrolytes In Solid-State Batteries

C. Rosenbach, F. Walther, J. Ruhl, M. Hartmann, T. A. Hendriks, S. Ohno, J. Janek, W. G. Zeier

Advanced Energy Materials, 2023, 13 (6), 2203673 DOI: 10.1002/aenm.202203673

Effect Of Particle Size And Pressure On The Transport Properties Of The Fast Ion Conductor t-Li₇SiPS₈

C. Schneider, C. P. Schmidt, A. Neumann, M. Clausnitzer, M. Sadowski, S. Harm, C. Meier, T. Danner, K. Albe, A. Latz, W. A. Wall, B. V. Lotsch

Advanced Energy Materials, 2023, 13 (15), 2203873 DOI: 10.1002/aenm.202203873

Mitigating Contact Loss In Li₆PS₅Cl-Based Solid-State Batteries Using A Thin Cationic Polymer Coating On NCM

B. Shi, Y. Yusim, S. Sen, T. Demuth, R. Ruess, K. Volz, A. Henss, F. H. Richter

Advanced Energy Materials, 2023, 13 (24), 2300310 DOI: 10.1002/aenm.202300310

Data-Driven Virtual Material Analysis And Synthesis For Solid Electrolyte Interphases

D. Rajagopal, A. Koeppe, M. Esmaeilpour, M. Selzer, W. Wenzel, H. Stein, B. Nestler

Advanced Energy Materials, 2023, 13 (40), 2301985 DOI: 10.1002/aenm.202301985

Kinetics And Pore Formation Of The Sodium Metal Anode On Nasicon-Type Na_3.4Zr₂Si_2.4P_0.6O₁₂ For Sodium Solid-State Batteries

T. Ortmann, S. Burkhardt, J. K. Eckhardt, T. Fuchs, Z. Ding, J. Sann, M. Rohnke, Q. Ma, F. Tietz, D. Fattakhova-Rohlfing, C. Kübel, O. Guillon, C. Heiliger, J. Janek

Advanced Energy Materials, 2023, 13 (5), 2202712 DOI: 10.1002/aenm.202202712

2D Layered Nanomaterials As Fillers In Polymer Composite Electrolytes For Lithium Batteries

V. Vijayakumar, M. Ghosh, K. Asokan, S. B. Sukumaran, S. Kurungot, J. Mindemark, D. Brandell, M. Winter, J. R. Nair

Advanced Energy Materials, 2023, 13 (15), 2203326 DOI: 10.1002/aenm.202203326

A Roadmap For Solid-State Batteries

T. Schmaltz, F. Hartmann, T. Wicke, L. Weymann, C. Neef, J. Janek

Advanced Energy Materials, 2023, 13 (43), 2301886 DOI: 10.1002/aenm.202301886

In Situ Observation Of Room-Temperature Magnesium Metal Deposition On A Nasicon/IL Hybrid Solid Electrolyte

Z. Wei, D. K. Singh, K. Helmbrecht, J. Sann, Y. Yusim, J. A. Kieser, C. Glaser, M. Rohnke, A. Groß, J. Janek

Advanced Energy Materials, 2023, 2302525 DOI: 10.1002/aenm.202302525

Characterization Of Porous Membranes Using Artificial Neural Networks

Y. Zhao, P. Altschuh, J. Santoki, L. Griem, G. Tosato, M. Selzer, A. Koeppe, B. Nestler

Acta Materialia, 2023, 253, 118922 DOI: 10.1016/j.actamat.2023.118922

Aqueous Processing Of LiCoO₂–Li_6.6La₃Zr_1.6Ta_0.4O₁₂ Composite Cathode For High-Capacity Solid-State Lithium Batteries

R. Ye, M. Ihrig, E. Figgemeier, D. Fattakhova-Rohlfing, M. Finsterbusch

ACS Sustainable Chemistry & Engineering, 2023, 11 (13), 5184-5194 DOI: 10.1021/acssuschemeng.2c07556

Single-Ion Conducting Multi-Block Copolymer Electrolyte For Lithium-Metal Batteries With High Mass Loading NCM811 Cathodes

X. Dong, A. Mayer, X. Liu, S. Passerini, D. Bresser

ACS Energy Letters, 2023, 8 (2), 1114-1121 DOI: 10.1021/acsenergylett.2c02806

Influence Of Microstructure On The Material Properties Of LLZO Ceramics Derived By Impedance Spectroscopy And Brick Layer Model Analysis

J. K. Eckhardt, S. Kremer, T. Fuchs, P. Minnmann, J. Schubert, S. Burkhardt, M. T. Elm, P. J. Klar, C. Heiliger, J. Janek

ACS Applied Materials & Interfaces, 2023, 15 (40), 47260-47277 DOI: 10.1021/acsami.3c10060

Identification Of Lithium Compounds On Surfaces Of Lithium Metal Anode With Machine-Learning-Assisted Analysis Of ToF-SIMS Spectra

Y. Zhao, S. Otto, T. Lombardo, A. Henss, A. Koeppe, M. Selzer, J. Janek, B. Nestler

ACS Applied Materials & Interfaces, 2023, 15 (43), 50469-50478 DOI: 10.1021/acsami.3c09643

Selection Of Polymer Segment Species Matters For Electrolyte Properties And Performance In Lithium Metal Batteries

M. Chiou, E. Verweyen, D. Diddens, L. Wichmann, C. Schmidt, K. Neuhaus, A. Choudhary, D. Bedrov, M. Winter, G. Brunklaus

ACS Applied Energy Materials, 2023, 6 (8), 4422-4436 DOI: 10.1021/acsaem.3c00571

Dissolution And Recrystallization Behavior Of Li₃PS₄ In Different Organic Solvents With A Focus On N-Methylformamide

K. Wissel, L. M. Riegger, C. Schneider, A. I. Waidha, T. Famprikis, Y. Ikeda, B. Grabowski, R. E. Dinnebier, B. V. Lotsch, J. Janek, W. Ensinger, O. Clemens

ACS Applied Energy Materials, 2023, 6 (15), 7790-7802 DOI: 10.1021/acsaem.2c03278

Structure Determination Of The Crystalline LiPON Model Structure Li_5+XP₂O_6−XN_1+X With X≈0.9

S. Schneider, L. G. Balzat, B. V. Lotsch, W. Schnick

Chemistry – A European Journal, 2023, 29 (9), e202202984 DOI: 10.1002/chem.202202984

Comprehensive Investigation Of Anion Species In Crystalline Li⁺ Ion Conductor Li_27−X[P₄O_7+XN_9−X]O₃ (X≈1.9(3))

S. Schneider, E. Wendinger, V. Baran, A. Hatz, B. V. Lotsch, M. Nentwig, O. Oeckler, T. Bräuniger, W. Schnick

Chemistry – A European Journal, 2023, 29 (27), e202300174 DOI: 10.1002/chem.202300174

2022

Embracing Disorder In Solid-State Batteries

M. Botros, J. Janek

Science, 2022, 378 (6626), 1273-1274 DOI: 10.1126/science.adf3383

Generating FAIR Research Data In Experimental Tribology

N. T. Garabedian, P. J. Schreiber, N. Brandt, P. Zschumme, I. L. Blatter, A. Dollmann, C. Haug, D. Kümmel, Y. Li, F. Meyer, C. E. Morstein, J. S. Rau, M. Weber, J. Schneider, P. Gumbsch, M. Selzer, C. Greiner

Scientific Data, 2022, 9 (1), 315 DOI: 10.1038/s41597-022-01429-9

Characterization Of Stressing Conditions In A High Energy Ball Mill By Discrete Element Simulations

C. F. Burmeister, M. Hofer, P. Molaiyan, P. Michalowski, A. Kwade

Processes, 2022, 10 (4), 692 DOI: 10.3390/pr10040692

Sintering Of Li-Garnets: Impact Of Al-Incorporation And Powder-Bed Composition On Microstructure And Ionic Conductivity

S. Lobe, A. Bauer, D. Sebold, N. Wettengl, D. Fattakhova-Rohlfing, S. Uhlenbruck

Open Ceramics, 2022, 10, 100268 DOI: 10.1016/j.oceram.2022.100268

NaSICON-Type Solid-State Li⁺ Ion Conductors With Partial Polyanionic Substitution Of Phosphate With Silicate

A. Loutati, O. Guillon, F. Tietz, D. Fattakhova-Rohlfing

Open Ceramics, 2022, 12, 100313 DOI: 10.1016/j.oceram.2022.100313

A Machine-Learned Interatomic Potential For Silica And Its Relation To Empirical Models

L. C. Erhard, J. Rohrer, K. Albe, V. L. Deringer

npj Computational Materials, 2022, 8 (1), 90 DOI: 10.1038/s41524-022-00768-w

High Areal Capacity, Long Cycle Life 4 V Ceramic All-Solid-State Li-Ion Batteries Enabled By Chloride Solid Electrolytes

L. Zhou, T. Zuo, C. Y. Kwok, S. Y. Kim, A. Assoud, Q. Zhang, J. Janek, L. F. Nazar

Nature Energy, 2022, 7 (1), 83-93 DOI: 10.1038/s41560-021-00952-0

Li-Ion Conductive Li_1.3Al_0.3Ti_1.7(PO₄)₃ (LATP) Solid Electrolyte Prepared By Cold Sintering Process With Various Sintering Additives

M. Vinnichenko, K. Waetzig, A. Aurich, C. Baumgaertner, M. Herrmann, C. W. Ho, M. Kusnezoff, C. W. Lee

Nanomaterials, 2022, 12 (18), 3178 DOI: 10.3390/nano12183178

Photo-Cross-Linked Single-Ion Conducting Polymer Electrolyte For Lithium-Metal Batteries

H. Liang, Z. Chen, X. Dong, T. Zinkevich, S. Indris, S. Passerini, D. Bresser

Macromolecular Rapid Communications, 2022, 43 (12), 2100820 DOI: 10.1002/marc.202100820

Green Polymer Electrolytes Based On Polycaprolactones For Solid-State High-Voltage Lithium Metal Batteries

Y. Chen, Y. Hsieh, K. L. Liu, L. Wichmann, J. H. Thienenkamp, A. Choudhary, D. Bedrov, M. Winter, G. Brunklaus

Macromolecular Rapid Communications, 2022, 43 (20), 2200335 DOI: 10.1002/marc.202200335

Single-Ion Conducting Polymer Electrolyte For Li||LiNi_0.6Mn_0.2Co_0.2O₂ Batteries—Impact Of The Anodic Cutoff Voltage And Ambient Temperature

D. Steinle, Z. Chen, H. Nguyen, M. Kuenzel, C. Iojoiu, S. Passerini, D. Bresser

Journal of Solid State Electrochemistry, 2022, 26 (1), 97-102 DOI: 10.1007/s10008-020-04895-6

Guidelines To Correctly Measure The Lithium Ion Conductivity Of Oxide Ceramic Electrolytes Based On A Harmonized Testing Procedure

M. Müller, H. Auer, A. Bauer, S. Uhlenbruck, M. Finsterbusch, K. Wätzig, K. Nikolowski, S. Dierickx, D. Fattakhova-Rohlfing, O. Guillon, A. Weber

Journal of Power Sources, 2022, 531, 231323 DOI: 10.1016/j.jpowsour.2022.231323

Durable Fast-Charging Lithium Metal Batteries Designed With Cross-Linked Polymer Electrolytes And Niobate-Coated Cathode

M. Chiou, K. Borzutzki, J. H. Thienenkamp, M. Mohrhardt, K. Liu, V. Mereacre, J. R. Binder, H. Ehrenberg, M. Winter, G. Brunklaus

Journal of Power Sources, 2022, 538, 231528 DOI: 10.1016/j.jpowsour.2022.231528

Quantifying Lithium Enrichment At Grain Boundaries In Li₇La₃Zr₂O₁₂ Solid Electrolyte By Correlative Microscopy

O. Cojocaru-Mirédin, J. Schmieg, M. Müller, A. Weber, E. Ivers-Tiffée, D. Gerthsen

Journal of Power Sources, 2022, 539, 231417 DOI: 10.1016/j.jpowsour.2022.231417

Rapid Thermal Processing Of Garnet-Based Composite Cathodes

W. S. Scheld, S. Lobe, C. Dellen, M. Ihrig, G. Häuschen, L. C. Hoff, M. Finsterbusch, S. Uhlenbruck, O. Guillon, D. Fattakhova-Rohlfing

Journal of Power Sources, 2022, 545, 231872 DOI: 10.1016/j.jpowsour.2022.231872

The Effects Of Aluminum Concentration On The Microstructural And Electrochemical Properties Of Lithium Lanthanum Zirconium Oxide

A. C. Moy, G. Häuschen, D. Fattakhova-Rohlfing, J. B. Wolfenstine, M. Finsterbusch, J. Sakamoto

Journal of Materials Chemistry A, 2022, 10, 21955-21972 DOI: 10.1039/D2TA03676B

Free Standing Dual Phase Cathode Tapes – Scalable Fabrication And Microstructure Optimization Of Garnet-Based Ceramic Cathodes

M. Rosen, M. Finsterbusch, O. Guillon, D. Fattakhova-Rohlfing

Journal of Materials Chemistry A, 2022, 10 (5), 2320-2326 DOI: 10.1039/D1TA07194G

Conductivity Enhancement Of Al- And Ta-Substituted Li₇La₃Zr₂O₇ Solid Electrolytes By Nanoparticles

A. Bauer, M. Y. Ali, H. Orthner, S. Uhlenbruck, H. Wiggers, D. Fattakhova-Rohlfing, O. Guillon

Journal of the European Ceramic Society, 2022, 42 (3), 1033-1041 DOI: 10.1016/j.jeurceramsoc.2021.11.029

Transition Metal Oxides And Li₂CO₃ As Precursors For The Synthesis Of Ni-Rich Single-Crystalline NCM For Sustainable Lithium-Ion Battery Production

R. Ruess, M. A. Ulherr, E. Trevisanello, S. Schröder, A. Henss, J. Janek

Journal of The Electrochemical Society, 2022, 169 (7), 70531 DOI: 10.1149/1945-7111/ac8242

Deeper Understanding Of The Lithiation Reaction During The Synthesis Of LiNiO₂ Towards An Increased Production Throughput

P. Kurzhals, F. Riewald, M. Bianchini, S. Ahmed, A. M. Kern, F. Walther, H. Sommer, K. Volz, J. Janek

Journal of The Electrochemical Society, 2022, 169 (5), 50526 DOI: 10.1149/1945-7111/ac6c0b

Anhydrous LiNbO₃ Synthesis And Its Application For Surface Modification Of Garnet Type Li-Ion Conductors

M. Mann, C. Schwab, M. Ihrig, M. Finsterbusch, M. Martin, O. Guillon, D. Fattakhova-Rohlfing

Journal of The Electrochemical Society, 2022, 169 (4), 40564 DOI: 10.1149/1945-7111/ac6836

Influence Of Lithium Ion Kinetics, Particle Morphology And Voids On The Electrochemical Performance Of Composite Cathodes For All-Solid-State Batteries

A. Bielefeld, D. A. Weber, R. Rueß, V. Glavas, J. Janek

Journal of The Electrochemical Society, 2022, 169 (2), 20539 DOI: 10.1149/1945-7111/ac50df

A Coupled Finite Element Approach To Spatially Resolved Lithium Plating And Stripping In Three-Dimensional Anode Microstructures Of Lithium-Ion Cells

R. Fang, C. P. Schmidt, W. A. Wall

Journal of Computational Physics, 2022, 461, 111179 DOI: 10.1016/j.jcp.2022.111179

Digestion Processes And Elemental Analysis Of Oxide And Sulfide Solid Electrolytes

T. F. Malkowski, E. D. Boeding, D. Fattakhova-Rohlfing, N. Wettengl, M. Finsterbusch, G. M. Veith

Ionics, 2022, 28 (7), 3223-3231 DOI: 10.1007/s11581-022-04536-0

The Influence Of Hafnium Impurities On The Electrochemical Performance Of Tantalum Substituted Li₇La₃Zr₂O₁₂ Solid Electrolytes

M. Mann, M. Küpers, G. Häuschen, M. Finsterbusch, D. Fattakhova-Rohlfing, O. Guillon

Ionics, 2022, 28 (1), 53-62 DOI: 10.1007/s11581-021-04300-w

Explainable Artificial Intelligence For Mechanics: Physics-Explaining Neural Networks For Constitutive Models

A. Koeppe, F. Bamer, M. Selzer, B. Nestler, B. Markert

Frontiers in Materials, 2022, 8, DOI: 10.3389/fmats.2021.824958

Machine Learning Assisted Design Of Experiments For Solid State Electrolyte Lithium Aluminum Titanium Phosphate

Y. Zhao, N. Schiffmann, A. Koeppe, N. Brandt, E. C. Bucharsky, K. G. Schell, M. Selzer, B. Nestler

Frontiers in Materials, 2022, 9, DOI: 10.3389/fmats.2022.821817

Novel Sulfur-Doped Single-Ion Conducting Multi-Block Copolymer Electrolyte

A. Mayer, T. Ates, A. Varzi, S. Passerini, D. Bresser

Frontiers in Chemistry, 2022, 10, DOI: 10.3389/fchem.2022.974202

KadiStudio: Fair Modelling Of Scientific Research Processes

L. Griem, P. Zschumme, M. Laqua, N. Brandt, E. Schoof, P. Altschuh, M. Selzer

Data Science Journal, 2022, 21 (1), 16 DOI: 10.5334/dsj-2022-016

Managing FAIR Tribological Data Using Kadi4Mat

N. Brandt, N. T. Garabedian, E. Schoof, P. J. Schreiber, P. Zschumme, C. Greiner, M. Selzer

Data, 2022, 7 (2), 15 DOI: 10.3390/data7020015

Effect Of Particle Size And Pressure On The Transport Properties Of The Fast Ion Conductor t-Li₇SiPS₈

C. Schneider, C. P. Schmidt, A. Neumann, M. Clausnitzer, M. Sadowski, S. Harm, C. Meier, T. Danner, K. Albe, A. Latz, W. A. Wall, B. V. Lotsch

ChemRxiv, 2022, DOI: 10.26434/chemrxiv-2022-tvc6l

The Impact Of Lithium Tungstate On The Densification And Conductivity Of Phosphate Lithium-Ion Conductors

P. Odenwald, Q. Ma, B. Davaasuren, E. Dashjav, F. Tietz, M. Wolff, W. Rheinheimer, S. Uhlenbruck, O. Guillon, D. Fattakhova-Rohlfing

ChemElectroChem, 2022, 9 (5), e202101366 DOI: 10.1002/celc.202101366

Correlating Structural Disorder To Li⁺ Ion Transport In Li_4–XGe_1–XSb_xS4 (0 ≤ X ≤ 0.2)

B. Helm, N. Minafra, B. Wankmiller, M. T. Agne, C. Li, A. Senyshyn, M. R. Hansen, W. G. Zeier

Chemistry of Materials, 2022, 34 (12), 5558-5570 DOI: 10.1021/acs.chemmater.2c00608

Instability Of The Li₇SiPS₈ Solid Electrolyte At The Lithium Metal Anode And Interphase Formation

L. M. Riegger, S. Otto, M. Sadowski, S. Jovanovic, O. Kötz, S. Harm, L. G. Balzat, S. Merz, S. Burkhardt, F. H. Richter, J. Sann, R. Eichel, B. V. Lotsch, J. Granwehr, K. Albe, J. Janek

Chemistry of Materials, 2022, 34 (8), 3659-3669 DOI: 10.1021/acs.chemmater.1c04302

Enhancing Ionic Conductivity By In Situ Formation Of Li₇SiPS₈/Argyrodite Hybrid Solid Electrolytes

R. Calaminus, S. Harm, D. H. Fabini, L. G. Balzat, A. Hatz, V. Duppel, I. Moudrakovski, B. V. Lotsch

Chemistry of Materials, 2022, 34 (17), 7666-7677 DOI: 10.1021/acs.chemmater.2c00346

Li₆PS₅Cl Microstructure And Influence On Dendrite Growth In Solid-State Batteries With Lithium Metal Anode

D. K. Singh, A. Henss, B. Mogwitz, A. Gautam, J. Horn, T. Krauskopf, S. Burkhardt, J. Sann, F. H. Richter, J. Janek

Cell Reports Physical Science, 2022, 3 (9), 101043 DOI: 10.1016/j.xcrp.2022.101043

Current Status Of Formulations And Scalable Processes For Producing Sulfidic Solid-State Batteries

M. Batzer, C. Heck, P. Michalowski, A. Kwade

Batteries & Supercaps, 2022, 5 (12), e202200328 DOI: 10.1002/batt.202200328

Survey Of Zirconium-Containing Nasicon-Type Solid-State Li⁺ Ion Conductors With The Aim Of Increasing Reduction Stability By Partial Cation Substitution

A. Loutati, P. Odenwald, B. Aktekin, J. Sann, O. Guillon, F. Tietz, D. Fattakhova-Rohlfing

Batteries & Supercaps, 2022, 5 (11), e202200327 DOI: 10.1002/batt.202200327

Ionic Liquid-Incorporated Metal-Organic Framework With High Magnesium Ion Conductivity For Quasi-Solid-State Magnesium Batteries

Z. Wei, R. Maile, L. M. Riegger, M. Rohnke, K. Müller-Buschbaum, J. Janek

Batteries & Supercaps, 2022, 5 (12), e202200318 DOI: 10.1002/batt.202200318

Dissolution And Recrystallization Behavior Of Li₃PS₄ In Different Organic Solvents

K. Wissel, L. M. Riegger, C. Schneider, A. I. Waidha, T. Famprikis, Y. Ikeda, B. Grabowski, R. E. Dinnebier, B. V. Lotsch, J. Janek, W. Ensinger, O. Clemens

arXiv, 2022, arXiv:2209.13955, DOI: 10.48550/arXiv.2209.13955

Structured Data Storage For Data-Driven Process Optimisation In Bioprinting

B. Schmieg, N. Brandt, V. J. Schnepp, L. Radosevic, S. Gretzinger, M. Selzer, J. Hubbuch

Applied Sciences, 2022, 12 (15), 7728 DOI: 10.3390/app12157728

In Situ Investigation Of Lithium Metal–Solid Electrolyte Anode Interfaces With Tof-Sims

S. Otto, L. M. Riegger, T. Fuchs, S. Kayser, P. Schweitzer, S. Burkhardt, A. Henss, J. Janek

Advanced Materials Interfaces, 2022, 9 (13), 2102387 DOI: 10.1002/admi.202102387

A Dry-Processed Al₂O₃/LiAlO₂ Coating For Stabilizing The Cathode/Electrolyte Interface In High-Ni NCM-Based All-Solid-State Batteries

R. S. Negi, Y. Yusim, R. Pan, S. Ahmed, K. Volz, R. Takata, F. Schmidt, A. Henss, M. T. Elm

Advanced Materials Interfaces, 2022, 9 (8), 2101428 DOI: 10.1002/admi.202101428

Designing Cathodes And Cathode Active Materials For Solid-State Batteries

P. Minnmann, F. Strauss, A. Bielefeld, R. Ruess, P. Adelhelm, S. Burkhardt, S. L. Dreyer, E. Trevisanello, H. Ehrenberg, T. Brezesinski, F. H. Richter, J. Janek

Advanced Energy Materials, 2022, 12 (35), 2201425 DOI: 10.1002/aenm.202201425

Polysiloxane-Based Single-Ion Conducting Polymer Blend Electrolyte Comprising Small-Molecule Organic Carbonates For High-Energy And High-Power Lithium-Metal Batteries

H. Liang, M. Zarrabeitia, Z. Chen, S. Jovanovic, S. Merz, J. Granwehr, S. Passerini, D. Bresser

Advanced Energy Materials, 2022, 12 (16), 2200013 DOI: 10.1002/aenm.202200013

Enhancing The Dendrite Tolerance Of Nasicon Electrolytes By Suppressing Edge Growth Of Na Electrode Along Ceramic Surface

Q. Ma, T. Ortmann, A. Yang, D. Sebold, S. Burkhardt, M. Rohnke, F. Tietz, D. Fattakhova-Rohlfing, J. Janek, O. Guillon

Advanced Energy Materials, 2022, 12 (40), 2201680 DOI: 10.1002/aenm.202201680

Influence Of Polymer Backbone Fluorination On The Electrochemical Behavior Of Single-Ion Conducting Multiblock Copolymer Electrolytes

A. Mayer, H. Nguyen, A. Mariani, T. Diemant, S. Lyonnard, C. Iojoiu, S. Passerini, D. Bresser

ACS Macro Letters, 2022, 11 (8), 982-990 DOI: 10.1021/acsmacrolett.2c00292

Silicon As Emerging Anode In Solid-State Batteries

H. Huo, J. Janek

ACS Energy Letters, 2022, 7 (11), 4005-4016 DOI: 10.1021/acsenergylett.2c01950

Superionic Conduction In The Plastic Crystal Polymorph Of Na₄P₂S₆

T. Scholz, C. Schneider, M. W. Terban, Z. Deng, R. Eger, M. Etter, R. E. Dinnebier, P. Canepa, B. V. Lotsch

ACS Energy Letters, 2022, 7 (4), 1403-1411 DOI: 10.1021/acsenergylett.1c02815

3D Impedance Modeling Of Metal Anodes In Solid-State Batteries–Incompatibility Of Pore Formation And Constriction Effect In Physical-Based 1D Circuit Models

J. K. Eckhardt, T. Fuchs, S. Burkhardt, P. J. Klar, J. Janek, C. Heiliger

ACS Applied Materials & Interfaces, 2022, 14 (37), 42757-42769 DOI: 10.1021/acsami.2c12991

Ceramic-In-Polymer Hybrid Electrolytes With Enhanced Electrochemical Performance

G. M. Overhoff, M. Y. Ali, J. Brinkmann, P. Lennartz, H. Orthner, M. Hammad, H. Wiggers, M. Winter, G. Brunklaus

ACS Applied Materials & Interfaces, 2022, 14 (48), 53636-53647 DOI: 10.1021/acsami.2c13408

Single-Ion Versus Dual-Ion Conducting Electrolytes: The Relevance Of Concentration Polarization In Solid-State Batteries

L. Stolz, S. Hochstädt, S. Röser, M. R. Hansen, M. Winter, J. Kasnatscheew

ACS Applied Materials & Interfaces, 2022, 14 (9), 11559-11566 DOI: 10.1021/acsami.2c00084

Does Cell Polarization Matter In Single-Ion Conducting Electrolytes?

K. Borzutzki, J. R. Nair, M. Winter, G. Brunklaus

ACS Applied Materials & Interfaces, 2022, 14 (4), 5211-5222 DOI: 10.1021/acsami.1c19097

Reducing Impedance At A Li-Metal Anode/Garnet-Type Electrolyte Interface Implementing Chemically Resolvable In Layers

M. Müller, J. Schmieg, S. Dierickx, J. Joos, A. Weber, D. Gerthsen, E. Ivers-Tiffée

ACS Applied Materials & Interfaces, 2022, 14 (12), 14739-14752 DOI: 10.1021/acsami.1c25257

All-Solid-State Li Batteries With NCM–Garnet-Based Composite Cathodes: The Impact Of NCM Composition On Material Compatibility

C. Roitzheim, Y. J. Sohn, L. Kuo, G. Häuschen, M. Mann, D. Sebold, M. Finsterbusch, P. Kaghazchi, O. Guillon, D. Fattakhova-Rohlfing

ACS Applied Energy Materials, 2022, 5 (6), 6913-6926 DOI: 10.1021/acsaem.2c00533

Can Substitutions Affect The Oxidative Stability Of Lithium Argyrodite Solid Electrolytes?

A. Banik, Y. Liu, S. Ohno, Y. Rudel, A. Jiménez-Solano, A. Gloskovskii, N. M. Vargas-Barbosa, Y. Mo, W. G. Zeier

ACS Applied Energy Materials, 2022, 5 (2), 2045-2053 DOI: 10.1021/acsaem.1c03599

Advanced Analytical Characterization Of Interface Degradation In Ni-Rich Ncm Cathode Co-Sintered With Latp Solid Electrolyte

M. Malaki, A. Pokle, S. Otto, A. Henss, J. P. Beaupain, A. Beyer, J. Müller, B. Butz, K. Wätzig, M. Kusnezoff, J. Janek, K. Volz

ACS Applied Energy Materials, 2022, 5 (4), 4651-4663 DOI: 10.1021/acsaem.2c00084

2021

From Ionic To Superionic Conductivity: The Influence Of Cation Order On Sodium Diffusion In Na₃Zr₂Si₂PO₁₂

L. Haarmann, K. Albe

Solid State Ionics, 2021, 363, 115604 DOI: 10.1016/j.ssi.2021.115604

Garnet To Hydrogarnet: Effect Of Post Synthesis Treatment On Cation Substituted LLZO Solid Electrolyte And Its Effect On Li Ion Conductivity

C. Fritsch, T. Zinkevich, S. Indris, M. Etter, V. Baran, T. Bergfeldt, M. Knapp, H. Ehrenberg, A. Hansen

RSC Advances, 2021, 11 (48), 30283-30294 DOI: 10.1039/D1RA05961K

Workflow Concepts To Model Nonlinear Mechanics With Computational Intelligence

A. Koeppe, F. Bamer, M. Selzer, B. Nestler, B. Markert

Proceedings in Applied Mathematics and Mechanics, 2021, 21 (1), e202100238 DOI: 10.1002/pamm.202100238

The Power Of Architecture – Cage -Shaped PEO And Its Application As A Polymer Electrolyte

A. Johannes Butzelaar, M. Gauthier-Jaques, K. Ling Liu, G. Brunklaus, M. Winter, P. Theato

Polymer Chemistry, 2021, 12 (30), 4326-4331 DOI: 10.1039/D1PY00490E

Block Copolymers As (Single-Ion Conducting) Lithium Battery Electrolytes

A. Mayer, D. Steinle, S. Passerini, D. Bresser

Nanotechnology, 2021, 33 (6), 62002 DOI: 10.1088/1361-6528/ac2e21

A Robust Technique To Image All Elements In LiNiO₂ Cathode Active Material By 4D-Stem

S. Ahmed, A. Pokle, J. Belz, M. Bianchini, A. Beyer, J. Janek, K. Volz

Microscopy and Microanalysis, 2021, 27 (S1), 1446-1449 DOI: 10.1017/S1431927621005353

Understanding The Formation Of Antiphase Boundaries In Layered Oxide Cathode Materials And Their Evolution Upon Electrochemical Cycling

S. Ahmed, A. Pokle, M. Bianchini, S. Schweidler, A. Beyer, T. Brezesinski, J. Janek, K. Volz

Matter, 2021, 4 (12), 3953-3966 DOI: 10.1016/j.matt.2021.10.001

Operando Analysis Of The Molten Li|LLZO Interface: Understanding How The Physical Properties Of Li Affect The Critical Current Density

B. Kinzer, A. L. Davis, T. Krauskopf, H. Hartmann, W. S. LePage, E. Kazyak, J. Janek, N. P. Dasgupta, J. Sakamoto

Matter, 2021, 4 (6), 1947-1961 DOI: 10.1016/j.matt.2021.04.016

The Sand Equation And Its Enormous Practical Relevance For Solid-State Lithium Metal Batteries

L. Stolz, G. Homann, M. Winter, J. Kasnatscheew

Materials Today, 2021, 44, 41883 DOI: 10.1016/j.mattod.2020.11.025

Realizing Poly(Ethylene Oxide) As A Polymer For Solid Electrolytes In High Voltage Lithium Batteries Via Simple Modification Of The Cell Setup

L. Stolz, G. Homann, M. Winter, J. Kasnatscheew

Materials Advances, 2021, 2 (10), 3251-3256 DOI: 10.1039/D1MA00009H

Evaluation Of Scalable Synthesis Methods For Aluminum-Substituted Li₇La₃Zr₂O₁₂ Solid Electrolytes

M. Mann, M. Küpers, G. Häuschen, M. Finsterbusch, D. Fattakhova-Rohlfing, O. Guillon

Materials, 2021, 14 (22), 6809 DOI: 10.3390/ma14226809

Polymer Electrolytes In Strong External Electric Fields: Modification Of Structure And Dynamics

A. Wettstein, D. Diddens, A. Heuer

Macromolecules, 2021, 54 (5), 2256-2265 DOI: 10.1021/acs.macromol.0c02385

Advanced Block Copolymer Design For Polymer Electrolytes: Prospects Of Microphase Separation

A. J. Butzelaar, P. Röring, M. Hoffmann, J. Atik, E. Paillard, M. Wilhelm, M. Winter, G. Brunklaus, P. Theato

Macromolecules, 2021, 54 (23), 11101-11112 DOI: 10.1021/acs.macromol.1c02147

Synthesis And Post-Polymerization Modification Of Defined Functional Poly(Vinyl Ether)s

A. J. Butzelaar, S. Schneider, E. Molle, P. Theato

Macromolecular Rapid Communications, 2021, 42 (13), 2100133 DOI: 10.1002/marc.202100133

Quasi-Solid Single Ion Conducting Polymer Electrolyte Membrane Containing Novel Fluorinated Poly(Arylene Ether Sulfonimide) For Lithium Metal Batteries

C. H. Krause, A. J. Butzelaar, D. Diddens, D. Dong, P. Théato, D. Bedrov, B. Hwang, M. Winter, G. Brunklaus

Journal of Power Sources, 2021, 484, 229267 DOI: 10.1016/j.jpowsour.2020.229267

Pragmatic Approaches To Correlate Between The Physicochemical Properties Of A Linear Poly(Ethylene Oxide)-Based Solid Polymer Electrolyte And The Performance In A High-Voltage Li-Metal Battery

L. Stolz, S. Röser, G. Homann, M. Winter, J. Kasnatscheew

The Journal of Physical Chemistry C, 2021, 125 (33), 18089-18097 DOI: 10.1021/acs.jpcc.1c03614

Impact Of Charged Surfaces On The Structure And Dynamics Of Polymer Electrolytes: Insights From Atomistic Simulations

A. Thum, D. Diddens, A. Heuer

The Journal of Physical Chemistry C, 2021, 125 (46), 25392-25403 DOI: 10.1021/acs.jpcc.1c07751

Computational Study Of The Structure Of Ternary Ionic Liquid/Salt/Polymer Electrolytes Based On Protic Ionic Liquids

J. M. Otero-Mato, A. Rivera-Pousa, H. Montes-Campos, O. Cabeza, A. Heuer, D. Diddens, L. M. Varela

Journal of Molecular Liquids, 2021, 333, 115883 DOI: 10.1016/j.molliq.2021.115883

Impact Of Hydration On Ion Transport In Li₂Sn₂S₅ · x H ₂ O

M. Joos, C. Schneider, A. Münchinger, I. Moudrakovski, R. Usiskin, J. Maier, B. V. Lotsch

Journal of Materials Chemistry A, 2021, 9 (30), 16532-16544 DOI: 10.1039/D1TA04736A

Controlling The Lithium Proton Exchange Of LLZO To Enable Reproducible Processing And Performance Optimization

M. Rosen, R. Ye, M. Mann, S. Lobe, M. Finsterbusch, O. Guillon, D. Fattakhova-Rohlfing

Journal of Materials Chemistry A, 2021, 9 (8), 4831-4840 DOI: 10.1039/D0TA11096E

Phase Formation Through Synthetic Control: Polymorphism In The Sodium-Ion Solid Electrolyte Na₄P₂S₆

T. Scholz, C. Schneider, R. Eger, V. Duppel, I. Moudrakovski, A. Schulz, J. Nuss, B. V. Lotsch

Journal of Materials Chemistry A, 2021, 9 (13), 8692-8703 DOI: 10.1039/D0TA11008F

Li₇La₃Zr₂O₁₂ Solid Electrolyte Sintered By The Ultrafast High-Temperature Method

M. Ihrig, T. P. Mishra, W. S. Scheld, G. Häuschen, W. Rheinheimer, M. Bram, M. Finsterbusch, O. Guillon

Journal of the European Ceramic Society, 2021, 41 (12), 6075-6079 DOI: 10.1016/j.jeurceramsoc.2021.05.041

Understanding The Impact Of Microstructure On Charge Transport In Polycrystalline Materials Through Impedance Modelling

J. K. Eckhardt, S. Burkhardt, J. Zahnow, M. T. Elm, J. Janek, P. J. Klar, C. Heiliger

Journal of The Electrochemical Society, 2021, 168 (9), 90516 DOI: 10.1149/1945-7111/ac1cfe

Editors’ Choice—Quantifying The Impact Of Charge Transport Bottlenecks In Composite Cathodes Of All-Solid-State Batteries

P. Minnmann, L. Quillman, S. Burkhardt, F. H. Richter, J. Janek

Journal of The Electrochemical Society, 2021, 168 (4), 40537 DOI: 10.1149/1945-7111/abf8d7

Editors’ Choice—Quantification Of The Impact Of Chemo-Mechanical Degradation On The Performance And Cycling Stability Of NCM-Based Cathodes In Solid-State Li-Ion Batteries

G. Conforto, R. Ruess, D. Schröder, E. Trevisanello, R. Fantin, F. H. Richter, J. Janek

Journal of The Electrochemical Society, 2021, 168 (7), 70546 DOI: 10.1149/1945-7111/ac13d2

Increasing The Lithium Ion Mobility In Poly(Phosphazene)-Based Solid Polymer Electrolytes Through Tailored Cation Doping

T. T. K. Ingber, D. Liebenau, M. Biedermann, M. Kolek, D. Diddens, H. Wiemhöfer, A. Heuer, M. Winter, P. Bieker

Journal of The Electrochemical Society, 2021, 168 (7), 70559 DOI: 10.1149/1945-7111/ac148d

rs@md: Introducing Reactive Steps At The Molecular Dynamics Simulation Level

M. Biedermann, D. Diddens, A. Heuer

Journal of Chemical Theory and Computation, 2021, 17 (2), 1074-1085 DOI: 10.1021/acs.jctc.0c01189

Upscaling Of LATP Synthesis: Stoichiometric Screening Of Phase Purity And Microstructure To Ionic Conductivity Maps

N. Schiffmann, E. C. Bucharsky, K. G. Schell, C. A. Fritsch, M. Knapp, M. J. Hoffmann

Ionics, 2021, 27 (5), 2017-2025 DOI: 10.1007/s11581-021-03961-x

Sn Substitution In The Lithium Superionic Argyrodite Li₆PCh₅I (Ch = S And Se)

A. Gautam, M. Ghidiu, A. Hansen, S. Ohno, W. G. Zeier

Inorganic Chemistry, 2021, 60 (24), 18975-18980 DOI: 10.1021/acs.inorgchem.1c02813

In Situ Polymerization Process: An Essential Design Tool For Lithium Polymer Batteries

V. Vijayakumar, B. Anothumakkool, S. Kurungot, M. Winter, J. Ravi Nair

Energy & Environmental Science, 2021, 14 (5), 2708-2788 DOI: 10.1039/D0EE03527K

Kadi4Mat: A Research Data Infrastructure For Materials Science

N. Brandt, L. Griem, C. Herrmann, E. Schoof, G. Tosato, Y. Zhao, P. Zschumme, M. Selzer

Data Science Journal, 2021, 20, 45146 DOI: 10.5334/dsj-2021-008

Kinetical Threshold Limits In Solid-State Lithium Batteries: Data On Practical Relevance Of Sand Equation

L. Stolz, G. Homann, M. Winter, J. Kasnatscheew

Data in Brief, 2021, 34, 106688 DOI: 10.1016/j.dib.2020.106688

Area Oversizing Of Lithium Metal Electrodes In Solid-State Batteries: Relevance For Overvoltage And Thus Performance?

L. Stolz, G. Homann, M. Winter, J. Kasnatscheew

ChemSusChem, 2021, 14 (10), 2163-2169 DOI: 10.1002/cssc.202100213

Order-Disorder Transition Driven Superionic Conduction In The New Plastic Polymorph Of Na₄P₂S₆

T. Scholz, C. Schneider, M. W. Terban, Z. Deng, R. Eger, M. Etter, R. E. Dinnebier, P. Canepa, B. V. Lotsch

ChemRxiv, 2021, DOI: 10.26434/chemrxiv-2021-7r31q

On The Underestimated Influence Of Synthetic Conditions In Solid Ionic Conductors

A. Banik, T. Famprikis, M. Ghidiu, S. Ohno, M. A. Kraft, W. G. Zeier

Chemical Science, 2021, 12 (18), 6238-6263 DOI: 10.1039/D0SC06553F

On The Additive Microstructure In Composite Cathodes And Alumina-Coated Carbon Microwires For Improved All-Solid-State Batteries

S. Randau, F. Walther, A. Neumann, Y. Schneider, R. S. Negi, B. Mogwitz, J. Sann, K. Becker-Steinberger, T. Danner, S. Hein, A. Latz, F. H. Richter, J. Janek

Chemistry of Materials, 2021, 33 (4), 1380-1393 DOI: 10.1021/acs.chemmater.0c04454

Synthesis And Postprocessing Of Single-Crystalline LiNi_0.8Co_0.15Al_0.05O₂ For Solid-State Lithium-Ion Batteries With High Capacity And Long Cycling Stability

R. Fantin, E. Trevisanello, R. Ruess, A. Pokle, G. Conforto, F. H. Richter, K. Volz, J. Janek

Chemistry of Materials, 2021, 33 (7), 2624-2634 DOI: 10.1021/acs.chemmater.1c00471

In-Depth Characterization Of Lithium-Metal Surfaces With XPS And ToF-SIMS: Toward Better Understanding Of The Passivation Layer

S. Otto, Y. Moryson, T. Krauskopf, K. Peppler, J. Sann, J. Janek, A. Henss

Chemistry of Materials, 2021, 33 (3), 859-867 DOI: 10.1021/acs.chemmater.0c03518

Stabilizing The Cathode/Electrolyte Interface Using A Dry-Processed Lithium Titanate Coating For All-Solid-State Batteries

R. S. Negi, P. Minnmann, R. Pan, S. Ahmed, M. J. Herzog, K. Volz, R. Takata, F. Schmidt, J. Janek, M. T. Elm

Chemistry of Materials, 2021, 33 (17), 6713-6723 DOI: 10.1021/acs.chemmater.1c01123

Fast Water-Assisted Lithium Ion Conduction In Restacked Lithium Tin Sulfide Nanosheets

A. Hatz, I. Moudrakovski, S. Bette, M. W. Terban, M. Etter, M. Joos, N. M. Vargas-Barbosa, R. E. Dinnebier, B. V. Lotsch

Chemistry of Materials, 2021, 33 (18), 7337-7349 DOI: 10.1021/acs.chemmater.1c01755

Lithium Deposition In Single-Ion Conducting Polymer Electrolytes

K. Borzutzki, K. Dong, J. R. Nair, B. Wolff, F. Hausen, R. Eichel, M. Winter, I. Manke, G. Brunklaus

Cell Reports Physical Science, 2021, 2 (7), 100496 DOI: 10.1016/j.xcrp.2021.100496

Working Principle Of An Ionic Liquid Interlayer During Pressureless Lithium Stripping On Li_6.25Al_0.25La₃Zr₂O₁₂ (LLZO) Garnet-Type Solid Electrolyte

T. Fuchs, B. Mogwitz, S. Otto, S. Passerini, F. H. Richter, J. Janek

Batteries & Supercaps, 2021, 4 (7), 1145-1155 DOI: 10.1002/batt.202100015

Pyridine Complexes As Tailored Precursors For Rapid Synthesis Of Thiophosphate Superionic Conductors

M. Ghidiu, R. Schlem, W. G. Zeier

Batteries & Supercaps, 2021, 4 (4), 607-611 DOI: 10.1002/batt.202000317

Absolute Local Quantification Of Li As Function Of State-Of-Charge In All-Solid-State Li Batteries Via 2D MeV Ion-Beam Analysis

S. Möller, T. Satoh, Y. Ishii, B. Teßmer, R. Guerdelli, T. Kamiya, K. Fujita, K. Suzuki, Y. Kato, H. Wiemhöfer, K. Mima, M. Finsterbusch

Batteries, 2021, 7 (2), 41 DOI: 10.3390/batteries7020041

Statics And Dynamics Of Space-Charge-Layers In Polarized Inorganic Solid Electrolytes

K. Becker-Steinberger, S. Schardt, B. Horstmann, A. Latz

arXiv, 2021, arXiv:2101.10294, DOI: 10.48550/arXiv.2101.10294

Lithium-Metal Anode Instability Of The Superionic Halide Solid Electrolytes And The Implications For Solid-State Batteries

L. M. Riegger, R. Schlem, J. Sann, W. G. Zeier, J. Janek

Angewandte Chemie International Edition, 2021, 60 (12), 6718-6723 DOI: 10.1002/anie.202015238

Polymorphism And Fast Potassium-Ion Conduction In The T5 Supertetrahedral Phosphidosilicate KSi₂P₃

A. Haffner, A. Hatz, O. E. O. Zeman, C. Hoch, B. V. Lotsch, D. Johrendt

Angewandte Chemie International Edition, 2021, 60 (24), 13641-13646 DOI: 10.1002/anie.202101187

Polymorphie Und Schnelle Kalium-Ionenleitung Im Phosphidosilicat KSi₂P₃ Mit T5 Supertetraedern

A. Haffner, A. Hatz, O. E. O. Zeman, C. Hoch, B. V. Lotsch, D. Johrendt

Angewandte Chemie, 2021, 133 (24), 13754-13759 DOI: 10.1002/ange.202101187

Physical Vapor Deposition In Solid-State Battery Development: From Materials To Devices

S. Lobe, A. Bauer, S. Uhlenbruck, D. Fattakhova-Rohlfing

Advanced Science, 2021, 8 (11), 2002044 DOI: 10.1002/advs.202002044

From Lithium-Metal Toward Anode-Free Solid-State Batteries: Current Developments, Issues, And Challenges

C. Heubner, S. Maletti, H. Auer, J. Hüttl, K. Voigt, O. Lohrberg, K. Nikolowski, M. Partsch, A. Michaelis

Advanced Functional Materials, 2021, 31 (51), 2106608 DOI: 10.1002/adfm.202106608

Lithium Phosphonate Functionalized Polymer Coating For High-Energy Li[Ni_0.8Co_0.1Mn_0.1]O2 With Superior Performance At Ambient And Elevated Temperatures

Z. Chen, H. Nguyen, M. Zarrabeitia, H. Liang, D. Geiger, J. Kim, U. Kaiser, S. Passerini, C. Iojoiu, D. Bresser

Advanced Functional Materials, 2021, 31 (41), 2105343 DOI: 10.1002/adfm.202105343

Impact Of Solvent Treatment Of The Superionic Argyrodite Li₆PS₅Cl On Solid-State Battery Performance

J. Ruhl, L. M. Riegger, M. Ghidiu, W. G. Zeier

Advanced Energy and Sustainability Research, 2021, 2 (2), 2000077 DOI: 10.1002/aesr.202000077

Engineering The Site-Disorder And Lithium Distribution In The Lithium Superionic Argyrodite Li₆PS₅Br

A. Gautam, M. Sadowski, M. Ghidiu, N. Minafra, A. Senyshyn, K. Albe, W. G. Zeier

Advanced Energy Materials, 2021, 11 (5), 2003369 DOI: 10.1002/aenm.202003369

Energy Storage Materials For Solid-State Batteries: Design By Mechanochemistry

R. Schlem, C. F. Burmeister, P. Michalowski, S. Ohno, G. F. Dewald, A. Kwade, W. G. Zeier

Advanced Energy Materials, 2021, 11 (30), 2101022 DOI: 10.1002/aenm.202101022

Lithium Argyrodite As Solid Electrolyte And Cathode Precursor For Solid-State Batteries With Long Cycle Life

S. Wang, M. Tang, Q. Zhang, B. Li, S. Ohno, F. Walther, R. Pan, X. Xu, C. Xin, W. Zhang, L. Li, Y. Shen, F. H. Richter, J. Janek, C. Nan

Advanced Energy Materials, 2021, 11 (31), 2101370 DOI: 10.1002/aenm.202101370

Influence Of Crystallinity Of Lithium Thiophosphate Solid Electrolytes On The Performance Of Solid-State Batteries

S. Wang, W. Zhang, X. Chen, D. Das, R. Ruess, A. Gautam, F. Walther, S. Ohno, R. Koerver, Q. Zhang, W. G. Zeier, F. H. Richter, C. Nan, J. Janek

Advanced Energy Materials, 2021, 11 (24), 2100654 DOI: 10.1002/aenm.202100654

A Systematic Study Of Vinyl Ether-Based Poly(Ethylene Oxide) Side-Chain Polymer Electrolytes

A. J. Butzelaar, K. L. Liu, P. Röring, G. Brunklaus, M. Winter, P. Theato

ACS Applied Polymer Materials, 2021, 3 (3), 1573-1582 DOI: 10.1021/acsapm.0c01398

Reaction Of Li_1.3Al_0.3Ti_1.7(PO₄)₃ And LiNi_0.6Co_0.2Mn_0.2O₂ In Co-Sintered Composite Cathodes For Solid-State Batteries

J. P. Beaupain, K. Waetzig, S. Otto, A. Henss, J. Janek, M. Malaki, A. Pokle, J. Müller, B. Butz, K. Volz, M. Kusnezoff, A. Michaelis

ACS Applied Materials & Interfaces, 2021, 13 (40), 47488-47498 DOI: 10.1021/acsami.1c11750

On The Origin Of Zero Interface Resistance In The Li_6.25Al_0.25La₃Zr₂O₁₂|Li⁰ System: An Atomistic Investigation

L. Haarmann, J. Rohrer, K. Albe

ACS Applied Materials & Interfaces, 2021, 13 (44), 52629-52635 DOI: 10.1021/acsami.1c15400

Styrene-Based Poly(Ethylene Oxide) Side-Chain Block Copolymers As Solid Polymer Electrolytes For High-Voltage Lithium-Metal Batteries

A. J. Butzelaar, P. Röring, T. P. Mach, M. Hoffmann, F. Jeschull, M. Wilhelm, M. Winter, G. Brunklaus, P. Théato

ACS Applied Materials & Interfaces, 2021, 13 (33), 39257-39270 DOI: 10.1021/acsami.1c08841

Storage Of Lithium Metal: The Role Of The Native Passivation Layer For The Anode Interface Resistance In Solid State Batteries

S. Otto, T. Fuchs, Y. Moryson, C. Lerch, B. Mogwitz, J. Sann, J. Janek, A. Henss

ACS Applied Energy Materials, 2021, 4 (11), 12798-12807 DOI: 10.1021/acsaem.1c02481

On The Lithium Distribution In Halide Superionic Argyrodites By Halide Incorporation In Li_7–XPS_6–XCl_x

A. Gautam, M. Ghidiu, E. Suard, M. A. Kraft, W. G. Zeier

ACS Applied Energy Materials, 2021, 4 (7), 7309-7315 DOI: 10.1021/acsaem.1c01417

Chemical Stability And Ionic Conductivity Of LGPS-Type Solid Electrolyte tetra-Li₇SiPS₈ After Solvent Treatment

A. Hatz, R. Calaminus, J. Feijoo, F. Treber, J. Blahusch, T. Lenz, M. Reichel, K. Karaghiosoff, N. M. Vargas-Barbosa, B. V. Lotsch

ACS Applied Energy Materials, 2021, 4 (9), 9932-9943 DOI: 10.1021/acsaem.1c01917

Analyzing Nanometer-Thin Cathode Particle Coatings For Lithium-Ion Batteries—The Example Of TiO2 On NCM622

Y. Moryson, F. Walther, J. Sann, B. Mogwitz, S. Ahmed, S. Burkhardt, L. Chen, P. J. Klar, K. Volz, S. Fearn, M. Rohnke, J. Janek

ACS Applied Energy Materials, 2021, 4 (7), 7168-7181 DOI: 10.1021/acsaem.1c01255

Influence Of Br⁻/S²⁻ Site-Exchange On Li Diffusion Mechanism In Li₆PS₅Br: A Computational Study

M. Sadowski, K. Albe

Philosophical Transactions of the Royal Society A: Mathematical, Physical and Engineering Sciences, 2021, 379 (2211), 20190458 DOI: 10.1098/rsta.2019.0458

2020

Transport Mechanism Of Lithium Ions In Non-Coordinating P(VdF-HFP) Copolymer Matrix

L. Mathies, D. Diddens, D. Dong, D. Bedrov, H. Leipner

Solid State Ionics, 2020, 357, 115497 DOI: 10.1016/j.ssi.2020.115497

Overcoming The Interfacial Limitations Imposed By The Solid–Solid Interface In Solid-State Batteries Using Ionic Liquid-Based Interlayers

S. A. Pervez, G. Kim, B. P. Vinayan, M. A. Cambaz, M. Kuenzel, M. Hekmatfar, M. Fichtner, S. Passerini

Small, 2020, 16 (14), 2000279 DOI: 10.1002/smll.202000279

An In Situ Cross-Linked Nonaqueous Polymer Electrolyte For Zinc-Metal Polymer Batteries And Hybrid Supercapacitors

V. Vijayakumar, M. Ghosh, M. Kurian, A. Torris, S. Dilwale, M. V. Badiger, M. Winter, J. R. Nair, S. Kurungot

Small, 2020, 16 (35), 2002528 DOI: 10.1002/smll.202002528

Poly(Ethylene Oxide)-Based Electrolyte For Solid-State-Lithium-Batteries With High Voltage Positive Electrodes: Evaluating The Role Of Electrolyte Oxidation In Rapid Cell Failure

G. Homann, L. Stolz, J. Nair, I. C. Laskovic, M. Winter, J. Kasnatscheew

Scientific Reports, 2020, 10 (1), 4390 DOI: 10.1038/s41598-020-61373-9

Application Of Random Forests In Tof-SIMS Data

Y. Zhao, S. Otto, N. Brandt, M. Selzer, B. Nestler

Procedia Computer Science, 2020, 176, 410-419 DOI: 10.1016/j.procs.2020.08.042

Solvate Ionic Liquids Based On Lithium Bis(Trifluoromethanesulfonyl)Imide–Glyme Systems: Coordination In MD Simulations With Scaled Charges

A. Thum, A. Heuer, K. Shimizu, J. N. C. Lopes

Physical Chemistry Chemical Physics, 2020, 22 (2), 525-535 DOI: 10.1039/C9CP04947A

Benchmarking The Performance Of All-Solid-State Lithium Batteries

S. Randau, D. A. Weber, O. Kötz, R. Koerver, P. Braun, A. Weber, E. Ivers-Tiffée, T. Adermann, J. Kulisch, W. G. Zeier, F. H. Richter, J. Janek

Nature Energy, 2020, 5 (3), 259-270 DOI: 10.1038/s41560-020-0565-1

High-Energy Lithium Batteries Based On Single-Ion Conducting Polymer Electrolytes And Li[Ni_0.8Co_0.1Mn_0.1]O₂ Cathodes

Z. Chen, D. Steinle, H. Nguyen, J. Kim, A. Mayer, J. Shi, E. Paillard, C. Iojoiu, S. Passerini, D. Bresser

Nano Energy, 2020, 77, 105129 DOI: 10.1016/j.nanoen.2020.105129

Recycling Strategies For Ceramic All-Solid-State Batteries—Part I: Study On Possible Treatments In Contrast To Li-Ion Battery Recycling

L. Schwich, M. Küpers, M. Finsterbusch, A. Schreiber, D. Fattakhova-Rohlfing, O. Guillon, B. Friedrich

Metals, 2020, 10 (11), 1523 DOI: 10.3390/met10111523

Computational Study Of Crystalline And Glassy Lithium Thiophosphates: Structure, Thermodynamic Stability And Transport Properties

M. Sadowski, K. Albe

Journal of Power Sources, 2020, 478, 229041 DOI: 10.1016/j.jpowsour.2020.229041

Understanding The Role Of Nanoparticles In Peo-Based Hybrid Polymer Electrolytes For Solid-State Lithium–Polymer Batteries

S. Nematdoust, R. Najjar, D. Bresser, S. Passerini

The Journal of Physical Chemistry C, 2020, 124 (51), 27907-27915 DOI: 10.1021/acs.jpcc.0c08749

High-Conductivity Free-Standing Li₆PS₅Cl/Poly(Vinylidene Difluoride) Composite Solid Electrolyte Membranes For Lithium-Ion Batteries

S. Wang, X. Zhang, S. Liu, C. Xin, C. Xue, F. Richter, L. Li, L. Fan, Y. Lin, Y. Shen, J. Janek, C. Nan

Journal of Materiomics, 2020, 6 (1), 70-76 DOI: 10.1016/j.jmat.2019.12.010

Improving The NMC111|Polymer Electrolyte Interface By Cathode Composition And Processing

K. Borzutzki, M. Winter, G. Brunklaus

Journal of The Electrochemical Society, 2020, 167 (7), 70546 DOI: 10.1149/1945-7111/ab7fb5

Elimination Of “Voltage Noise” Of Poly (Ethylene Oxide)-Based Solid Electrolytes In High-Voltage Lithium Batteries: Linear Versus Network Polymers

G. Homann, L. Stolz, M. Winter, J. Kasnatscheew

iScience, 2020, 23 (6), 101225 DOI: 10.1016/j.isci.2020.101225

Small Groups, Big Impact: Eliminating Li⁺ Traps In Single-Ion Conducting Polymer Electrolytes

K. Borzutzki, D. Dong, C. Wölke, M. Kruteva, A. Stellhorn, M. Winter, D. Bedrov, G. Brunklaus

iScience, 2020, 23 (8), 101417 DOI: 10.1016/j.isci.2020.101417

Finding The Right Blend: Interplay Between Structure And Sodium Ion Conductivity In The System Na₅AlS₄–Na₄SiS₄

S. Harm, A. Hatz, C. Schneider, C. Hoefer, C. Hoch, B. V. Lotsch

Frontiers in Chemistry, 2020, 8, DOI: 10.3389/fchem.2020.00090

Synthesis And Structure Of The Sodium Phosphidosilicate Na₂SiP₂

A. Haffner, A. Hatz, C. Hoch, B. V. Lotsch, D. Johrendt

European Journal of Inorganic Chemistry, 2020, 2020 (7), 617-621 DOI: 10.1002/ejic.201901083

From Liquid- To Solid-State Batteries: Ion Transfer Kinetics Of Heteroionic Interfaces

M. Weiss, F. J. Simon, M. R. Busche, T. Nakamura, D. Schröder, F. H. Richter, J. Janek

Electrochemical Energy Reviews, 2020, 3 (2), 221-238 DOI: 10.1007/s41918-020-00062-7

A Bilayer Polymer Electrolyte Encompassing Pyrrolidinium-Based RTIL For Binder-Free Silicon Few-Layer Graphene Nanocomposite Anodes For Li-Ion Battery

M. Falco, S. Palumbo, G. Lingua, L. Silvestri, M. Winter, R. Lin, V. Pellegrini, F. Bonaccorso, J. R. Nair, C. Gerbaldi

Electrochemistry Communications, 2020, 118, 106807 DOI: 10.1016/j.elecom.2020.106807

Mechanochemical Synthesis Of Amorphous And Crystalline Na₂P₂S₆ – Elucidation Of Local Structural Changes By X-Ray Total Scattering And NMR

C. Fritsch, A. Hansen, S. Indris, M. Knapp, H. Ehrenberg

Dalton Transactions, 2020, 49 (5), 1668-1673 DOI: 10.1039/C9DT04777H

Reduced Sintering Temperatures Of Li+ Conductive Li1.3Al0.3Ti1.7(Po4)3 Ceramics

K. Waetzig, C. Heubner, M. Kusnezoff

Crystals, 2020, 10 (5), 408 DOI: 10.3390/cryst10050408

Physicochemical Concepts Of The Lithium Metal Anode In Solid-State Batteries

T. Krauskopf, F. H. Richter, W. G. Zeier, J. Janek

Chemical Reviews, 2020, 120 (15), 7745-7794 DOI: 10.1021/acs.chemrev.0c00431

Structure And Diffusion Pathways In Li₆PS₅Cl Argyrodite From Neutron Diffraction, Pair-Distribution Function Analysis, And NMR

R. Schlenker, A. Hansen, A. Senyshyn, T. Zinkevich, M. Knapp, T. Hupfer, H. Ehrenberg, S. Indris

Chemistry of Materials, 2020, 32 (19), 8420-8430 DOI: 10.1021/acs.chemmater.0c02418

Partially Oxidized Cellulose Grafted With Polyethylene Glycol Mono-Methyl Ether (m-PEG) As Electrolyte Material For Lithium Polymer Battery

S. Nematdoust, R. Najjar, D. Bresser, S. Passerini

Carbohydrate Polymers, 2020, 240, 116339 DOI: 10.1016/j.carbpol.2020.116339

Effective Optimization Of High Voltage Solid-State Lithium Batteries By Using Poly(Ethylene Oxide)-Based Polymer Electrolyte With Semi-Interpenetrating Network

G. Homann, L. Stolz, K. Neuhaus, M. Winter, J. Kasnatscheew

Advanced Functional Materials, 2020, 30 (46), 2006289 DOI: 10.1002/adfm.202006289

Visualization Of Light Elements Using 4D Stem: The Layered-To-Rock Salt Phase Transition In LiNiO₂ Cathode Material

S. Ahmed, M. Bianchini, A. Pokle, M. S. Munde, P. Hartmann, T. Brezesinski, A. Beyer, J. Janek, K. Volz

Advanced Energy Materials, 2020, 10 (25), 2001026 DOI: 10.1002/aenm.202001026

How Certain Are The Reported Ionic Conductivities Of Thiophosphate-Based Solid Electrolytes? An Interlaboratory Study

S. Ohno, T. Bernges, J. Buchheim, M. Duchardt, A. K. Hatz, M. A. Kraft, H. Kwak, A. L. Santhosha, Z. Liu, N. Minafra, F. Tsuji, A. Sakuda, R. Schlem, S. Xiong, Z. Zhang, P. Adelhelm, H. Chen, A. Hayashi, Y. S. Jung, B. V. Lotsch, B. Roling, N. M. Vargas-Barbosa, W. G. Zeier

ACS Energy Letters, 2020, 5 (3), 910-915 DOI: 10.1021/acsenergylett.9b02764

Modeling Effective Ionic Conductivity And Binder Influence In Composite Cathodes For All-Solid-State Batteries

A. Bielefeld, D. A. Weber, J. Janek

ACS Applied Materials & Interfaces, 2020, 12 (11), 12821-12833 DOI: 10.1021/acsami.9b22788

Analysis Of Interfacial Effects In All-Solid-State Batteries With Thiophosphate Solid Electrolytes

A. Neumann, S. Randau, K. Becker-Steinberger, T. Danner, S. Hein, Z. Ning, J. Marrow, F. H. Richter, J. Janek, A. Latz

ACS Applied Materials & Interfaces, 2020, 12 (8), 9277-9291 DOI: 10.1021/acsami.9b21404

In Situ Monitoring Of Thermally Induced Effects In Nickel-Rich Layered Oxide Cathode Materials At The Atomic Level

A. Pokle, S. Ahmed, S. Schweidler, M. Bianchini, T. Brezesinski, A. Beyer, J. Janek, K. Volz

ACS Applied Materials & Interfaces, 2020, 12 (51), 57047-57054 DOI: 10.1021/acsami.0c16685

Interphase Formation Of PEO₂₀:LiTFSI–Li₆PS₅Cl Composite Electrolytes With Lithium Metal

F. J. Simon, M. Hanauer, F. H. Richter, J. Janek

ACS Applied Materials & Interfaces, 2020, 12 (10), 11713-11723 DOI: 10.1021/acsami.9b22968

Dioxolanone-Anchored Poly(Allyl Ether)-Based Cross-Linked Dual-Salt Polymer Electrolytes For High-Voltage Lithium Metal Batteries

V. Vijayakumar, D. Diddens, A. Heuer, S. Kurungot, M. Winter, J. R. Nair

ACS Applied Materials & Interfaces, 2020, 12 (1), 567-579 DOI: 10.1021/acsami.9b16348

Changing The Static And Dynamic Lattice Effects For The Improvement Of The Ionic Transport Properties Within The Argyrodite Li₆PS_5–XSe_xI

R. Schlem, M. Ghidiu, S. P. Culver, A. Hansen, W. G. Zeier

ACS Applied Energy Materials, 2020, 3 (1), 43344 DOI: 10.1021/acsaem.9b01794

2019

4-V Flexible All-Solid-State Lithium Polymer Batteries

Z. Chen, G. Kim, Z. Wang, D. Bresser, B. Qin, D. Geiger, U. Kaiser, X. Wang, Z. X. Shen, S. Passerini

Nano Energy, 2019, 64, 103986 DOI: 10.1016/j.nanoen.2019.103986

Decoupling Segmental Relaxation And Ionic Conductivity For Lithium-Ion Polymer Electrolytes

D. Bresser, S. Lyonnard, C. Iojoiu, L. Picard, S. Passerini

Molecular Systems Design & Engineering, 2019, 4 (4), 779-792 DOI: 10.1039/C9ME00038K

Solution-Based Synthesis Of Lithium Thiophosphate Superionic Conductors For Solid-State Batteries: A Chemistry Perspective

M. Ghidiu, J. Ruhl, S. P. Culver, W. G. Zeier

Journal of Materials Chemistry A, 2019, 7 (30), 17735-17753 DOI: 10.1039/C9TA04772G

Lithium Metal Polymer Electrolyte Batteries: Opportunities And Challenges

J. R. Nair, L. Imholt, G. Brunklaus, M. Winter

The Electrochemical Society Interface, 2019, 28 (2), 55 DOI: 10.1149/2.F05192if

A Crosslinked Polyethyleneglycol Solid Electrolyte Dissolving Lithium Bis(Trifluoromethylsulfonyl)Imide For Rechargeable Lithium Batteries

G. Tian, Z. Zhao, T. Zinkevich, K. Elies, F. Scheiba, H. Ehrenberg

ChemSusChem, 2019, 12 (20), 4708-4718 DOI: 10.1002/cssc.201901587

Rapid Crystallization And Kinetic Freezing Of Site-Disorder In The Lithium Superionic Argyrodite Li₆PS₅Br

A. Gautam, M. Sadowski, N. Prinz, H. Eickhoff, N. Minafra, M. Ghidiu, S. P. Culver, K. Albe, T. F. Fässler, M. Zobel, W. G. Zeier

Chemistry of Materials, 2019, 31 (24), 10178-10185 DOI: 10.1021/acs.chemmater.9b03852

Lesson Learned From NMR: Characterization And Ionic Conductivity Of LGPS-Like Li₇SiPS₈

S. Harm, A. Hatz, I. Moudrakovski, R. Eger, A. Kuhn, C. Hoch, B. V. Lotsch

Chemistry of Materials, 2019, 31 (4), 1280-1288 DOI: 10.1021/acs.chemmater.8b04051

The Role Of Intragranular Nanopores In Capacity Fade Of Nickel-Rich Layered Li(Ni_1–X–YCo_xMn_y)O₂ Cathode Materials

S. Ahmed, A. Pokle, S. Schweidler, A. Beyer, M. Bianchini, F. Walther, A. Mazilkin, P. Hartmann, T. Brezesinski, J. Janek, K. Volz

ACS Nano, 2019, 13 (9), 10694-10704 DOI: 10.1021/acsnano.9b05047

Properties Of The Interphase Formed Between Argyrodite-Type Li₆PS₅Cl And Polymer-Based PEO₁₀:LiTFSI

F. J. Simon, M. Hanauer, A. Henss, F. H. Richter, J. Janek

ACS Applied Materials & Interfaces, 2019, 11 (45), 42186-42196 DOI: 10.1021/acsami.9b14506

2018

Synthesis And Characterization Of Three New Lithium-Scandium Hexathiohypodiphosphates: Li_4–3XSc_xP₂S₆ (X = 0.358), m-LiScP₂S₆, And t-LiScP₂S₆

L. M. Schoop, R. Eger, F. Pielnhofer, C. Schneider, J. Nuss, B. V. Lotsch

Zeitschrift für anorganische und allgemeine Chemie, 2018, 644 (24), 1854-1862 DOI: 10.1002/zaac.201800363